843 research outputs found

    Electron-Hole Asymmetry in GdBaCo_{2}O_{5+x}: Evidence for Spin Blockade of Electron Transport in a Correlated Electron System

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    In RBaCo_{2}O_{5+x} compounds (R is rare earth) variability of the oxygen content allows precise doping of CoO_2 planes with both types of charge carriers. We study transport properties of doped GdBaCo_{2}O_{5+x} single crystals and find a remarkable asymmetry in the behavior of holes and electrons doped into a parent insulator GdBaCo_{2}O_{5.5}. Doping dependences of resistivity, Hall response, and thermoelectric power reveal that the doped holes greatly improve the conductivity, while the electron-doped samples always remain poorly conducting. This doping asymmetry provides strong evidence for a spin blockade of the electron transport in RBaCo_{2}O_{5+x}.Comment: 4 pages, 5 figures, accepted for publication in PR

    Quantum oscillations in a topological insulator Bi_{1-x}Sb_{x}

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    We have studied transport and magnetic properties of Bi_{1-x}Sb_x, which is believed to be a topological insulator - a new state of matter where an insulating bulk supports an intrinsically metallic surface. In nominally insulating Bi_{0.91}Sb_{0.09} crystals, we observed strong quantum oscillations of the magnetization and the resistivity originating from a Fermi surface which has a clear two-dimensional character. In addition, a three-dimensional Fermi surface is found to coexist, which is possibly due to an unusual coupling of the bulk to the surface. This finding demonstrates that quantum oscillations can be a powerful tool to directly probe the novel electronic states in topological insulators.Comment: 4 pages, 4 figure

    Additional Evidence for the Surface Origin of the Peculiar Angular-Dependent Magnetoresistance Oscillations Discovered in a Topological Insulator Bi_{1-x}Sb_{x}

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    We present detailed data on the unusual angular-dependent magnetoresistance oscillation phenomenon recently discovered in a topological insulator Bi_{0.91}Sb_{0.09}. Direct comparison of the data taken before and after etching the sample surface gives compelling evidence that this phenomenon is essentially originating from a surface state. The symmetry of the oscillations suggests that it probably comes from the (111) plane, and obviously a new mechanism, such as a coupling between the surface and the bulk states, is responsible for this intriguing phenomenon in topological insulators.Comment: 5 pages, 4 figures, Proceedings manuscript for the 19th International Conference on the Application of High Magnetic Fields in Semiconductor Physics and Nanotechnology (HMF-19

    Ising-like Spin Anisotropy and Competing Antiferromagnetic - Ferromagnetic Orders in GdBaCo_{2}O_{5.5} Single Crystals

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    In RBaCo_{2}O_{5+x} compounds (R is rare earth), a ferromagnetic-antiferromagnetic competition is accompanied by a giant magnetoresistance. We study the magnetization of detwinned GdBaCo_{2}O_{5.5} single crystals, and find a remarkable uniaxial anisotropy of Co^{3+} spins which is tightly linked with the chain oxygen ordering in GdO_{0.5} planes. Reflecting the underlying oxygen order, CoO_2 planes also develop a spin-state order consisting of Co^{3+} ions in alternating rows of S=1 and S=0 states. The magnetic structure appears to be composed of weakly coupled ferromagnetic ladders with Ising-like moments, which gives a simple picture for magnetotransport phenomena.Comment: 5 pages, 4 figures, accepted to Phys.Rev.Let

    Origin of the large thermoelectric power in oxygen-variable RBaCo_{2}O_{5+x} (R=Gd, Nd)

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    Thermoelectric properties of GdBaCo_{2}O_{5+x} and NdBaCo_{2}O_{5+x} single crystals have been studied upon continuous doping of CoO_2 planes with either electrons or holes. The thermoelectric response and the resistivity behavior reveal a hopping character of the transport in both compounds, providing the basis for understanding the recently found remarkable divergence of the Seebeck coefficient at x=0.5. The doping dependence of the thermoelectric power evinces that the configurational entropy of charge carriers, enhanced by their spin and orbital degeneracy, plays a key role in the origin of the large thermoelectric response in these correlated oxides.Comment: 5 pages, 4 figures, accepted for publication in PR
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