The Quantum Nature of a Nuclear Phase Transition

In their ground states, atomic nuclei are quantum Fermi liquids. At finite temperatures and low densities, these nuclei may undergo a phase change similar to, but substantially different from, a classical liquid gas phase transition. As in the classical case, temperature is the control parameter while density and pressure are the conjugate variables. At variance with the classical case, in the nucleus the difference between the proton and neutron concentrations acts as an additional order parameter, for which the symmetry potential is the conjugate variable. Different ratios of the neutron to proton concentrations lead to different critical points for the phase transition. This is analogous to the phase transitions occurring in $^{4}$He-$^{3}$He liquid mixtures. We present experimental results which reveal the N/Z dependence of the phase transition and discuss possible implications of these observations in terms of the Landau Free Energy description of critical phenomena.Comment: 5 pages, 4 figure

Isocaling and the Symmetry Energy in the Multifragmentation Regime of Heavy Ion Collisions

The ratio of the symmetry energy coefficient to temperature, $a_sym/T$, in Fermi energy heavy ion collisions, has been experimentally extracted as a function of the fragment atomic number using isoscaling parameters and the variance of the isotope distributions. The extracted values have been compared to the results of calculations made with an Antisymmetrized Molecular Dynamics (AMD) model employing a statistical decay code to account for deexcitation of excited primary fragments. The experimental values are in good agreement with the values calculated but are significantly different from those characterizing the yields of the primary AMD fragments.Comment: 12 pages, 6 figure

Critical behavior of the isotope yield distributions in the Multifragmentation Regime of Heavy Ion Reactions

Isotope yields have been analyzed within the framework of a Modified Fisher Model to study the power law yield distribution of isotopes in the multifragmentation regime. Using the ratio of the mass dependent symmetry energy coefficient relative to the temperature, $a_{sym}/T$, extracted in previous work and that of the pairing term, $a_{p}/T$, extracted from this work, and assuming that both reflect secondary decay processes, the experimentally observed isotope yields have been corrected for these effects. For a given I = N - Z value, the corrected yields of isotopes relative to the yield of $^{12}C$ show a power law distribution, $Y(N,Z)/Y(^{12}C) \sim A^{-\tau}$, in the mass range of $1 \le A \le 30$ and the distributions are almost identical for the different reactions studied. The observed power law distributions change systematically when I of the isotopes changes and the extracted $\tau$ value decreases from 3.9 to 1.0 as I increases from -1 to 3. These observations are well reproduced by a simple de-excitation model, which the power law distribution of the primary isotopes is determined to $\tau^{prim} = 2.4 \pm 0.2$, suggesting that the disassembling system at the time of the fragment formation is indeed at or very near the critical point.Comment: 5 pages, 5 figure

The Isospin Dependence Of The Nuclear Equation Of State Near The Critical Point

We discuss experimental evidence for a nuclear phase transition driven by the different concentration of neutrons to protons. Different ratios of the neutron to proton concentrations lead to different critical points for the phase transition. This is analogous to the phase transitions occurring in 4He-3He liquid mixtures. We present experimental results which reveal the N/A (or Z/A) dependence of the phase transition and discuss possible implications of these observations in terms of the Landau Free Energy description of critical phenomena.Comment: 14 pages, 18 figure

Isobaric Yield Ratios and The Symmetry Energy In Fermi Energy Heavy Ion Reactions

The relative isobaric yields of fragments produced in a series of heavy ion induced multifragmentation reactions have been analyzed in the framework of a Modified Fisher Model, primarily to determine the ratio of the symmetry energy coefficient to the temperature, $a_a/T$, as a function of fragment mass A. The extracted values increase from 5 to ~16 as A increases from 9 to 37. These values have been compared to the results of calculations using the Antisymmetrized Molecular Dynamics (AMD) model together with the statistical decay code Gemini. The calculated ratios are in good agreement with those extracted from the experiment. In contrast, the ratios determined from fitting the primary fragment distributions from the AMD model calculation are ~ 4 and show little variation with A. This observation indicates that the value of the symmetry energy coefficient derived from final fragment observables may be significantly different than the actual value at the time of fragment formation. The experimentally observed pairing effect is also studied within the same simulations. The Coulomb coefficient is also discussed.Comment: 10 pages, 12 figure

A novel approach to Isoscaling: the role of the order parameter m = (N-Z)/A

Isoscaling is derived within a recently proposed modified Fisher model where the free energy near the critical point is described by the Landau O(m^6) theory. In this model m = (N-Z)/A is the order parameter, a consequence of (one of) the symmetries of the nuclear Hamiltonian. Within this framework we show that isoscaling depends mainly on this order parameter through the 'external (conjugate) field' H. The external field is just given by the difference in chemical potentials of the neutrons and protons of the two sources. To distinguish from previously employed isoscaling relationships, this approach is dubbed: m - scaling. We discuss the relationship between this framework and the standard isoscaling formalism and point out some substantial differences in interpretation of experimental results which might result. These should be investigated further both theoretically and experimentally.Comment: 14 pages, 5 figure

Evidence of Critical Behavior in the Disassembly of Nuclei with A ~ 36

A wide variety of observables indicate that maximal fluctuations in the disassembly of hot nuclei with A ~ 36 occur at an excitation energy of 5.6 +- 0.5 MeV/u and temperature of 8.3 +- 0.5 MeV. Associated with this point of maximal fluctuations are a number of quantitative indicators of apparent critical behavior. The associated caloric curve does not appear to show a flattening such as that seen for heavier systems. This suggests that, in contrast to similar signals seen for liquid-gas transitions in heavier nuclei, the observed behavior in these very light nuclei is associated with a transition much closer to the critical point.Comment: v2: Major changes, new model calculations, new figure

Experimental reconstruction of primary hot isotopes and characteristic properties of the fragmenting source in the heavy ion reactions near the Fermi energy

The characteristic properties of the hot nuclear matter existing at the time of fragment formation in the multifragmentation events produced in the reaction $^{64}$Zn + $^{112}$Sn at 40 MeV/nucleon are studied. A kinematical focusing method is employed to determine the multiplicities of evaporated light particles, associated with isotopically identified detected fragments. From these data the primary isotopic yield distributions are reconstructed using a Monte Carlo method. The reconstructed yield distributions are in good agreement with the primary isotope distributions obtained from AMD transport model simulations. Utilizing the reconstructed yields, power distribution, Landau free energy, characteristic properties of the emitting source are examined. The primary mass distributions exhibit a power law distribution with the critical exponent, $A^{-2.3}$, for $A \geq 15$ isotopes, but significantly deviates from that for the lighter isotopes. Landau free energy plots show no strong signature of the first order phase transition. Based on the Modified Fisher Model, the ratios of the Coulomb and symmetry energy coefficients relative to the temperature, $a_{c}/T$ and $a_{sym}/T$, are extracted as a function of A. The extracted $a_{sym}/T$ values are compared with results of the AMD simulations using Gogny interactions with different density dependencies of the symmetry energy term. The calculated $a_{sym}/T$ values show a close relation to the symmetry energy at the density at the time of the fragment formation. From this relation the density of the fragmenting source is determined to be $\rho /\rho_{0} = (0.63 \pm 0.03 )$. Using this density, the symmetry energy coefficient and the temperature of fragmenting source are determined in a self-consistent manner as $a_{sym} = (24.7 \pm 3.4) MeV$ and $T=(4.9 \pm 0.2)$ MeV

Critical Behavior in Light Nuclear Systems: Experimental Aspects

An extensive experimental survey of the features of the disassembly of a small quasi-projectile system with $A \sim$ 36, produced in the reactions of 47 MeV/nucleon $^{40}$Ar + $^{27}$Al, $^{48}$Ti and $^{58}$Ni, has been carried out. Nuclei in the excitation energy range of 1-9 MeV/u have been investigated employing a new method to reconstruct the quasi-projectile source. At an excitation energy $\sim$ 5.6 MeV/nucleon many observables indicate the presence of maximal fluctuations in the de-excitation processes. The fragment topological structure shows that the rank sorted fragments obey Zipf's law at the point of largest fluctuations providing another indication of a liquid gas phase transition. The caloric curve for this system shows a monotonic increase of temperature with excitation energy and no apparent plateau. The temperature at the point of maximal fluctuations is $8.3 \pm 0.5$ MeV. Taking this temperature as the critical temperature and employing the caloric curve information we have extracted the critical exponents $\beta$, $\gamma$ and $\sigma$ from the data. Their values are also consistent with the values of the universality class of the liquid gas phase transition. Taken together, this body of evidence strongly suggests a phase change in an equilibrated mesoscopic system at, or extremely close to, the critical point.Comment: Physical Review C, in press; some discussions about the validity of excitation energy in peripheral collisions have been added; 24 pages and 32 figures; longer abstract in the preprin