Buoyancy driven bubbly flows: role of meso-scale structures on the relative motion between phases in bubble columns operated in the heterogeneous regime

The hydrodynamics of bubble columns in the heterogeneous regime is investigated from experiments with bubbles at large particle Reynolds numbers and without coalescence. The void fraction field $\varepsilon$ at small scales, analyzed with Vorono\"i tessellations, corresponds to a Random Poisson Process (RPP) in homogeneous conditions but it significantly differs from a RPP in the heterogeneous regime. The distance to a RPP allows identifying meso-scale structures, namely clusters, void regions and intermediate regions. A series of arguments demonstrate that the bubble motion is driven by the dynamics of these structures. Notably, bubbles in clusters (respectively in intermediate regions) are moving up faster, up to 3.5 (respectively 2) times the terminal velocity, than bubbles in void regions those absolute velocity equals the mean liquid velocity. Besides, the mean unconditional relative velocity of bubbles is recovered from mean relative velocities conditional to meso-scale structures, weighted by the proportion of bubbles in each structure. Assuming buoyancy-inertia equilibrium for each structure, the relative velocity is related with the characteristic size and concentration of meso-scale structures. By taking the latter quantities values at large gas superficial velocities, a cartoon of the internal flow structure is proposed. Arguments are put forward to help understanding why the relative velocity scales as $(gD\varepsilon)^{1/2}$ (with $D$ the column's diameter and $g$ gravity's acceleration). The proposed cartoon seems consistent with a fast-track mechanism that, for the moderate Rouse numbers studied, leads to liquid velocity fluctuations proportional to the relative velocity. The potential impact of coalescence on the above analysis is also commented.Comment: arXiv admin note: substantial text overlap with arXiv:2203.0741

Turbulent transport of material particles: An experimental study of finite size effects

We use an acoustic Lagrangian tracking technique, particularly adapted to measurements in open flows, and a versatile material particles generator (in the form of soap bubbles with adjustable size and density) to characterize Lagrangian statistics of finite sized, neutrally bouyant, particles transported in an isotropic turbulent flow of air. We vary the size of the particles in a range corresponding to turbulent inertial scales and explore how the turbulent forcing experienced by the particles depends on their size. We show that, while the global shape of the intermittent acceleration probability density function does not depend significantly on particle size, the acceleration variance of the particles decreases as they become larger in agreement with the classical scaling for the spectrum of Eulerian pressure fluctuations in the carrier flow

Measurement of gas phase characteristics using amonofibre optical probe in a three-phase flow

The study of gas–liquid–solid systems structure requires reliable measurement tools. In this paper, preliminary results on the potential use of a monofibre optical probe to investigate such flow are presented. This probe, manufactured at LEGI, allows the simultaneous measurement of the gas phase residence time and gas phase velocity. This specificity makes this probe more interesting than classical single tip probes (which measure only the gas residence time) or double tip probes (which are more intrusive). Although extensively used in two-phase gas–liquid, this probe was never used in gas–liquid–solid systems. First, the probe signal response is studied for three-phase flow conditions in the presence of solids. Results show that for soft solids, the probe tips can be contaminated when the probe pierces the solid. The signal processing procedure was modified accordingly to take into account these events. Second, the probe results are validated by comparing global results (global void fraction, gas flowrate) deduced from profile measurements with measurements performed by independent means. Lastly, void fraction profiles and interfacial area are studied more in detail. Depending on the solid loading, these profiles exhibit different behaviours. These features are associated to characteristics of the flow such as the transition from an homogeneous regime to an heterogenous regime, and are consistent with global observation performed by independent means. This demonstrates the ability of the probe to connect local information to the global behaviour and structure of the flow.Fundação para a Ciência e a Tecnologia (FCT

Customization of an optical probe device and validation of a signal processing procedure to study gas-liquid-solid flows. Application to a three-phase internal-loop Gas-lift Bioreactor

The study of local hydrodynamic properties of three-phase bioreactors in biotechnology processes is of great importance, mainly because of the complex interaction between bioreactor and microorganisms. However, classical techniques used for measuring local hydrodynamic properties such as single needle probes are mainly limited to two-phase flows. In this work it was developed and validated a new system, based on the customization of an optical probe initially designed in LEGI. The necessity of a new system was due to the agglomeration of the solid-phase (spent grains which are used as the micro-organisms carrier for the targeted application) around the optical tip, which influences the measurements. This new system allows for the measurement of the main local gas-phase properties in a complex gas-liquid-solid mixture. The new system was first validated for air-water system in an internal loop gas-lift reactor and then applied to a spent grains-air-water mixture at low solid load in an internal gas lift reactor. In addition, experiments using complementary techniques (as high speed camera and PIV) were performed that allowed for the validation of the new system and the explanation of possible physical mechanisms that are underlying on this multiphase system. The system developed has the potential for improvement and use in several biotechnology applications.The authors gratefully acknowledge the financial support from FCT (Fundacao para a Ciencia e Tecnologia, SFRH/BD/37082/2007 and SFRH/BPD/45637/2008)

Characteristics of clustered particles in skimming flows on a stepped spillway

Air–water flows at hydraulic structures are commonly observed and called white waters. The free-surface aeration is characterised by some intense exchanges of air and water leading to complex air–water structures including some clustering. The number and properties of clusters may provide some measure of the level of particle-turbulence and particle–particle interactions in the high-velocity air–water flows. Herein a re-analysis of air–water clusters was applied to a highly aerated free-surface flow data set (Chanson and Carosi, Exp Fluids 42:385–401, 2007). A two-dimensional cluster analysis was introduced combining a longitudinal clustering criterion based on near-wake effect and a side-by-side particle detection method. The results highlighted a significant number of clustered particles in the high-velocity free-surface flows. The number of bubble/droplet clusters per second and the percentage of clustered particles were significantly larger using the two-dimensional cluster analysis than those derived from earlier longitudinal detection techniques only. A number of large cluster structures were further detected. The results illustrated the complex interactions between entrained air and turbulent structures in skimming flow on a stepped spillway, and the cluster detection method may apply to other highly aerated free-surface flows

O2 mass transfer in an oscillatory flow reactor provided with smooth periodic constrictions : individual characterization of kL and a

In the present work the superficial gas velocities ( u G ) and the oscillatory conditions (frequency and amplitude) effects on the gas–liquid mass transfer process in a novel oscillatory flow reactor provided with smooth periodic constrictions (OFR-SPC) are experimentally evaluated. The liquid-side mass transfer coefficient, k L , and the specific interfacial area, a, are studied individually. The specific interfacial area is obtained using the new automatic image analysis technique developed by Ferreira et al. (2012). The experimental results of volumetric liquid side mass transfer coefficient ( k L a ), Sauter mean diameter ( d 32 ) and gas holdup ( ε G ), and the calculated values of a and k L , are correlated with the superficial gas velocity and the power density ( P / V ), in order to be used in scale-up processes and in comparisons with the literature. The results show that k L a increases with both superficial gas velocity and oscillatory conditions, the last ones having the highest impact on the mass transfer process. The increase in the oscillation motion (frequency and amplitude) results in bubble size reduction (from ∼7 mm, without oscillation, to ∼1 mm, with oscillation), in bubble average residence time increase and, consequently, in a increase. A k L increase with d 32 decrease is observed, showing the importance of hydrodynamic phenomena on k L , specially, when very low bubbles sizes are presented in oscillatory flow reactors.This work was supported by Fundacao para a Ciencia e Tecnologia under program contract number SFRH/BPD/45637/2008