Dipolar Interactions in Superconductor-Ferromagnet Heterostructures

We consider a simple model for a superlattice composed of a thin magnetic film placed between two bulk superconductors. The magnetic film is modelled by a planar but otherwise arbitrary distribution of magnetic dipoles and the superconductors are treated in the London approximation. Due to the linearity of the problem, we are able to compute the magnetic energy of the film in the presence of the superconductors. We show that in the case of small wavenumbers compared to the inverse London penetration depth, the magnetic energy resembles the energy of a distribution of magnetisation in a two dimensional space. Possible experimental applications of these results are discussed.Comment: RevTeX, 29 pages, 3 figures. To be published in Phys. Rev. B. Changes were made (including adding fig. 3), to conform with the referee's report. Reference 54 was also adde

Fundamental limits to optical response in absorptive systems

At visible and infrared frequencies, metals show tantalizing promise for strong subwavelength resonances, but material loss typically dampens the response. We derive fundamental limits to the optical response of absorptive systems, bounding the largest enhancements possible given intrinsic material losses. Through basic conservation-of-energy principles, we derive geometry-independent limits to per-volume absorption and scattering rates, and to local-density-of-states enhancements that represent the power radiated or expended by a dipole near a material body. We provide examples of structures that approach our absorption and scattering limits at any frequency, by contrast, we find that common "antenna" structures fall far short of our radiative LDOS bounds, suggesting the possibility for significant further improvement. Underlying the limits is a simple metric, $|\chi|^2 / \operatorname{Im} \chi$ for a material with susceptibility $\chi$, that enables broad technological evaluation of lossy materials across optical frequencies.Comment: 21 pages and 6 figures (excluding appendices, references

Model for quantitative tip-enhanced spectroscopy and the extraction of nanoscale-resolved optical constants

Near-field infrared spectroscopy by elastic scattering of light from a probe tip resolves optical contrasts in materials at dramatically sub-wavelength scales across a broad energy range, with the demonstrated capacity for chemical identification at the nanoscale. However, current models of probe-sample near-field interactions still cannot provide a sufficiently quantitatively interpretation of measured near-field contrasts, especially in the case of materials supporting strong surface phonons. We present a model of near-field spectroscopy derived from basic principles and verified by finite-element simulations, demonstrating superb predictive agreement both with tunable quantum cascade laser near-field spectroscopy of SiO$_2$ thin films and with newly presented nanoscale Fourier transform infrared (nanoFTIR) spectroscopy of crystalline SiC. We discuss the role of probe geometry, field retardation, and surface mode dispersion in shaping the measured near-field response. This treatment enables a route to quantitatively determine nano-resolved optical constants, as we demonstrate by inverting newly presented nanoFTIR spectra of an SiO$_2$ thin film into the frequency dependent dielectric function of its mid-infrared optical phonon. Our formalism further enables tip-enhanced spectroscopy as a potent diagnostic tool for quantitative nano-scale spectroscopy.Comment: 19 pages, 9 figure

Nonlinear resonance reflection from and transmission through a dense glassy system built up of oriented linear Frenkel chains: two-level models

A theoretical study of the resonance optical response of assemblies of oriented short (as compared to an optical wavelength) linear Frenkel chains is carried out using a two-level model. We show that both transmittivity and reflectivity of the film may behave in a bistable fashion and analyze how the effects found depend on the film thickness and on the inhomogeneous width of the exciton optical transition.Comment: 26 pages, 9 figure