Silica bottle resonator sensor for refractive index and temperature measurements

We propose and theoretically demonstrate a bottle resonator sensor with a nanoscale altitude and with alength several of hundreds of microns made on the top of the fiber with a radius of tens microns for refractive index and temperature sensor applications. The whispering gallery modes (WGMs) in the resonators can be excited with a taper fiber placed on the top of the resonator. These sensors can be considered as an alternative to fiber Bragg grating (FBG) sensors.The sensitivity of TM-polarized modes is higher than the sensitivity of the TE-polarized modes, but these values are comparable and both polarizations are suitable for sensor applications. The sensitivity similar to 150 (nm/RIU) can be reached with abottle resonator on the fiber with the radius 10 m. It can be improved with theuse of a fiber with a smaller radius. The temperature sensitivity is found to be similar to 10 pm/K. The temperature sensitivity can decrease similar to 10% for a fiber with a radius r(co) = 10 m instead of a fiber with a radius r(co) = 100 m. These sensors have sensitivities comparable to FBG sensors. A bottle resonator sensor with a nanoscale altitude made on the top of the fiber can be easily integrated in any fiber scheme

Novel Sensing Mechanisms for Chemical and Bio-sensing Using Whispering Gallery Mode Microresonators

Due to their ultra-high quality factor and small mode volume, whispering gallery mode (WGM) microresonators have proven to have exceptional sensing capabilities, with single particle level sensitivity to virions, proteins, and nucleic acids. Current sensing mechanisms rely on measuring the changes in the transmission spectrum of the resonator upon adsorption of the analyte on the surface of the resonator, appearing as either shift, splitting, or broadening of the resonance mode, all of which measure the polarizability of adsorbed analytes. In this dissertation, we present two new sensing mechanisms for WGM microresonators: the measurement of a dynamic chemical reaction around the resonator, exemplified by the polymerization of hydrogel, and the Raman spectroscopy of molecules on the surface of WGM microresonator through WGM-based surface-enhanced Raman scattering. Further, an on-going work on sensing using mesoporous silica micro-bottle resonator is described in the last chapter. Our work on the measurement of gelation of polyacrylamide hydrogel using WGM resonators is the first report of using WGM resonators to continuously monitor a chemical reaction (i.e. gelation) in situ. The results from WGM sensing is compared with rheology, a well-established technique for hydrogel characterization. From the similarities and differences in the measured results from WGM and rheology, we suggest that whereas rheology measures the viscoelastic properties of the hydrogel, WGM resonators measure the hydrogel density indirectly through its refractive index. The two techniques provide data that complement each other, which can be used to study the gelation reaction in more details. Raman spectroscopy is a powerful technique for molecular fingerprinting, but the weak Raman signal often requires enhancement from techniques such as surface-enhanced Raman scattering (SERS). Conventionally, metallic nanostructures are used for SERS, but recently there has been increasing interest in the enhancement of Raman scattering from dielectric substrates due to their improved stability and biocompatibility compared with metallic substrates. The combination of WGM resonator and Raman spectroscopy can be a promising sensing platform with both high sensitivity and specificity. Here, we demonstrate the enhanced Raman scattering from rhodamine 6G molecules coated on silica microspheres, excited through WGMs. A total Raman enhancement factor of 1.4 × 104 is observed

Nanostructured optical fibre tapers and related applications

In the last decade, optical fibre tapers have attracted considerable interest because they offer a variety of enabling properties, including large evanescent fields, flexibility, configurability, high confinement, robustness and compactness. These distinctive features have been exploited in a wealth of applications ranging from telecommunication devices to sensors, from optical manipulation to high-Q resonators. Nanostructures on the optical fibre tapers are very promising since the size of the device can be extremely small. With the development of nanostructuring methods, sub-wavelength feature sizes have been achieved. In this thesis, nanostructured optical fibre tapers and some related applications are discussed.Light confinement is limited by diffraction and the minimum spot size is related to the light wavelength. In this thesis, light confinement in two and three dimensions is proposed and achieved with two typologies of nanostructured optical fibre tapers. The first group of devices exploits plasmons excited at the optical fibre tips to obtain high transmissivity, and confine light to a sub-wavelength dimension. Optical fibre tips were designed according to numerical simulations and coated by a layer of gold; an extremely small aperture was then opened at the tip apex. The experimental characterization and simulation results showed their improved transmission efficiency (higher than 10-2) and thermal expansion measurements showed no shape changes could be detected within the accuracy of the system (~2 nm) for 9 mW injected powers. Effective confinements to 10 nm or smaller can be envisaged by decreasing the aperture size and slope angle. Application of this small spot size source can include scanning near-field optical microscope, optical recording, photolithography and bio-sensing.The second group achieves three dimensional light confinement exploiting a Fabry-Perot microcavity formed by a microfibre grating similar to those used in distributed feedback lasers. Microfibres were patterned using a Focused Ion Beam (FIB) system. In this structure, the microcavity provides longitudinal light confinement, whereas air dielectric guiding by the microfibre provides diffraction limited confinement in the other two dimensions. Due to the high refractive index contrast between silica and air, strong reflection can be obtained by only dozens of notches. This device can be used for a wide range of applications, e.g. sensing and triggered single-photon sources.Light confinement in nanostructured optical fibre tapers was exploited in a micrometric thermometer. A compact thermometer based on a broadband microfibre coupler tip showed a dynamic range spanning from room temperature to 1511ºC with a response time of tens of microseconds. This is the highest temperature measured with a silica optical fibre device. An average sensitivity of 11.96 pm/ºC was achieved for a coupler tip with ~2.5 µm diameter. A resolution of 0.66ºC was achieved for a coupler tip diameter of ~12.6 µm. Better resolution can be achieved with smaller size microfibre coupler tips.Optical fibre tapers are commonly used to couple light to selected resonator modes. Here FIB was used to inscribe microgrooves on optical Bottleneck Microresonator (BMR) surfaces to excite selected whispering gallery modes. By monitoring the transmission spectrum of the optical fibre taper, substantial spectral clean-up was obtained in appropriately scarred BMRs. Single high-Q mode operation can be achieved by either using two asymmetrical perpendicular scars or placing the grooves closer to the BMR centre, providing the potential for high performance sensors and other optical devices.Finally, strong three dimensional localization has been achieved in Plasmonic Slot Nano-Resonators (PSNRs) embedded in a gold-coated optical fibre tapers. Different shapes PSNRs, embedded in thin gold metal film coated plasmonic microfibre, were numerically investigated. The intensity enhancement (in excess of 106) and the resonance wavelength depend on both the PSNR and microfibre dimensions. Theoretically and experimentally, the transversal excitation of a rectangular PSNR embedded in a thin gold film coated plasmonic fibre tip was discussed for the first time, and showed high localization and strong enhancement (7.24×103). This device can find a wide range of applications such as surface-enhanced Raman scattering, optical filtering, spectroscopy and bio-sensing

Sensing of multiple parameters with whispering gallery mode optical fiber micro-resonators

Monitoring of multiple physical parameters, such as humidity, temperature, strain, concentrations of certain chemicals or gases in various environments is of great importance in many industrial applications both for minimizing adverse effects on human health as well as for maintaining production levels and quality of products. In this paper we demonstrate two different approaches to the design of multi-parametric sensors using coupled whispering gallery mode (WGM) optical fiber micro-resonators. In the first approach, a small array of micro-resonators is coupled to a single fiber taper, while in the second approach each of the micro-resonators within an array is coupled to a different tapered fiber section fabricated along the same fiber length. Simultaneous measurement of relative humidity and ammonia concentration in air is demonstrated with an array of two microspheres with different functional coatings coupled to a single fiber taper. Sensitivity to ammonia of 19.07 pm/ppm ammonia molecules and sensitivity to relative humidity of 1.07 pm/% RH have been demonstrated experimentally. In the second approach, an inline cascade of two cylindrical micro-resonators fabricated by coupling to multiple tapered sections along a single optical fiber is demonstrated for measurement of strain and temperature simultaneously. A strain sensitivity of 1.4 pm/με and temperature sensitivity of 330 pm/ºC have been demonstrated experimentally. Both the proposed sensing systems have the potential for increase of the number of microresonators within an array for sensing of a larger number of parameters allowing for reduction of the overall cost of sensing system

A Packaged Whispering Gallery Mode Strain Sensor Based on a Polymer Wire Cylindrical Micro Resonator

We propose a whispering gallery mode (WGM) strain sensor formed by a polymer-wire cylindrical micro resonator for strain measurement applications. WGMs are generated by evanescently coupling light into the polymer-wire resonator from a silica fiber taper fabricated by the micro heater brushing technique. Accurate and repeatable measurements of a strains up to one free spectral range (FSR) shift of the WGMs (corresponding to 0.33 % of the polymer-wire elongation, 3250 μɛ) are demonstrated experimentally with the proposed sensor. Practical packaging method for the proposed strain sensor on a glass microscope slide has also been realized making the sensor portable and easy to handle. The robustness of the packaged coupling system is confirmed by vibration tests. The performance of the packaged strain sensor is evaluated and compared with that for an unpackaged sensor

Optical Whispering Gallery Mode Cylindrical Micro-Resonator Devices for Sensing Applications

Whispering gallery mode (WGM) micro-resonators are devices attractive for many practical applications including optical sensing, micro-lasers, optical switches, tunable filters and many others. Their popularity is due to the high Q-factors and the exceptional sensitivity of their optical properties to the resonator’s size, refractive index as well the properties of the surrounding medium. The main focus of this thesis is on the cylindrical WGM micro-resonators due to the simplicity of their fabrication and light coupling that they offer in comparison with other WGM devices. At first, an in-depth experimental investigation of the WGM effect in different types of cylindrical micro-resonators was carried out in order to establish the influence of the resonator’s geometry and coupling conditions on the resulting WGM spectrum. As one of the outcomes of this study, a novel method for geometrical profiling of asymmetries in thin microfiber tapers with submicron accuracy has been proposed and demonstrated. The submicron accuracy of the proposed method has been verified by SEM studies. The method can be applied as a quality control tool in fabrication of microfiber based devices and sensors or for fine-tuning of microfiber fabrication setups. The study also resulted in better understanding of the optimum conditions for excitation of WGMs in cylindrical fiber resonators, the influence of the tilt angle between the micro-cylinder and the coupling fiber taper. A novel strain sensor formed by a polymer-wire cylindrical micro-resonator has been developed. Accurate and repeatable measurements of strain have been demonstrated experimentally with the proposed sensor for the upper range of limit of detection up to 3250 με. Practical packaging method for the proposed strain sensor on a glass microscope slide has also been realized making the sensor portable and easy to use. A study of thermo-optic tuning of the WGMs in a nematic liquid crystal-filled hollow cylindrical microresonator has been carried out. A simple and robust packaging has been realized with the proposed tunable device to ensure its stable and repeatable operation. The demonstrated thermo-optic method for the WGMs tuning is potentially useful for many tunable photonic devices. Two novel all-fiber magnetic-field sensors have been designed based on photonic crystal fibers infiltrated with a magnetic fluid and a ferronematic liquid crystal utilizing the magnetic field tunability of WGM resonances. The highest experimentally demonstrated magnetic field sensitivity was 110 pm/mT in the range of magnetic fields from 0 to 40 mT. Finally, a packaged inline cascaded optical micro-resonators (ICOMRs) design is proposed for coupling multiple micro-resonators to a single fiber and simultaneous sensing of multiple parameters (strain, temperature, humidity, or refractive index) at multiple points in space has been demonstrated. The proposed design principle can find applications in quasi-distributed sensing, optical coding, optical logic gates and wavelength division multiplexed optical communications systems

Free spectral range electrical tuning of a high quality on-chip microcavity

Reconfigurable photonic circuits have applications ranging from next-generation computer architectures to quantum networks, coherent radar and optical metamaterials. However, complete reconfigurability is only currently practical on millimetre-scale device footprints. Here, we overcome this barrier by developing an on-chip high quality microcavity with resonances that can be electrically tuned across a full free spectral range (FSR). FSR tuning allows resonance with any source or emitter, or between any number of networked microcavities. We achieve it by integrating nanoelectronic actuation with strong optomechanical interactions that create a highly strain-dependent effective refractive index. This allows low voltages and sub-nanowatt power consumption. We demonstrate a basic reconfigurable photonic network, bringing the microcavity into resonance with an arbitrary mode of a microtoroidal optical cavity across a telecommunications fibre link. Our results have applications beyond photonic circuits, including widely tuneable integrated lasers, reconfigurable optical filters for telecommunications and astronomy, and on-chip sensor networks.Comment: Main text: 7 pages, 3 figures. Supplementary information: 7 pages, 9 figure