EXPERIMENTAL TECHNIQUE TO MEASURE THORON GENERATION RATE OF BUILDING MATERIAL SAMPLES USING RAD7 DETECTOR

Thoron (220Rn) is the second most abundant radon isotope in our living environment. In some dwellings it is present in significant amount which calls for its identification and remediation. Indoor thoron originates mainly from building materials. In this work we have developed and tested an experimental technique to measure thoron generation rate in building material samples using RAD7 radon-thoron detector. The mathematical model of the measurement technique provides the thoron concentration response of RAD7 as a function of the sample thickness. For experimental validation of the technique an adobe building material sample was selected for measuring the thoron concentration at nineteen different sample thicknesses. Fitting the parameters of the model to the measurement results, both the generation rate and the diffusion length of thoron was estimated. We have also determined the optimal sample thickness for estimating the thoron generation rate from a single measurement

The imprint of thermally induced devolatilization phenomena on radon signal. Implications for the geochemical survey in volcanic areas

Thermal gradients due to magma dynamics in active volcanic areas may affect the emanating power of the substrate and the background level of radon signal. This is particularly effective in subvolcanic substrates where intense hydrothermal alteration and/or weathering processes generally form hydrous minerals, such as zeolites able to store and release great amounts of H2O (up to ∼25 wt.%) at relative low temperatures. To better understand the role played by thermally induced devolatilization reactions on the radon signal, a new experimental setup has been developed for measuring in real time the radon emission from a zeolitized volcanic tuff. Progressive dehydration phenomena with increasing temperature produce radon emissions two orders of magnitude higher than those measured during rock deformation, microfracturing and failure. In this framework, mineral devolatilization reactions can contribute significantly to produce radon emissions spatially heterogeneous and non-stationary in time, resulting in a transient state dictated by temperature gradients and the carrier effects of subsurface gases. Results from these experiments can be extrapolated to the temporal and spatial scales of magmatic processes, where the ascent of small magma batches from depth causes volatile release due to dehydration phenomena that increase the radon signal from the degassing host rock material

Investigation of radioactivity-induced backgrounds in EXO-200

The search for neutrinoless double-beta decay (0{\nu}{\beta}{\beta}) requires extremely low background and a good understanding of their sources and their influence on the rate in the region of parameter space relevant to the 0{\nu}{\beta}{\beta} signal. We report on studies of various {\beta}- and {\gamma}-backgrounds in the liquid- xenon-based EXO-200 0{\nu}{\beta}{\beta} experiment. With this work we try to better understand the location and strength of specific background sources and compare the conclusions to radioassay results taken before and during detector construction. Finally, we discuss the implications of these studies for EXO-200 as well as for the next-generation, tonne-scale nEXO detector.Comment: 9 pages, 7 figures, 3 table

Radon Daughter Plate-out onto Teflon

Radiopure materials for detector components in rare event searches may be contaminated after manufacturing with long-lived $^{210}$Pb produced by the decay of atmospheric radon. Charged radon daughters deposited on the surface or implanted in the bulk of detector materials have the potential to cause noticeable backgrounds within dark matter regions of interest. Understanding the mechanics governing these background signals is therefore a paramount concern in dark matter experiments in order to distinguish a real signal from internal detector backgrounds. Teflon ($i.e.$ PTFE) is a specific material of interest because it makes up the walls of the inner detector of many liquid noble detectors such as the LUX-ZEPLIN experiment. The rate of radon daughter plate-out onto Teflon can be orders of magnitude larger than the plate-out rate onto other materials. Mitigation of plate-out onto Teflon and steel by proximity to other materials is demonstrated.Comment: Low Radioactivity Techniques (LRT) Workshop 2017, 4 Pages, 5 Figure

Construction and measurements of a vacuum-swing-adsorption radon-mitigation system

Long-lived alpha and beta emitters in the $^{222}$Rn decay chain on (and near) detector surfaces may be the limiting background in many experiments attempting to detect dark matter or neutrinoless double-beta decay, and in screening detectors. In order to reduce backgrounds from radon-daughter plate-out onto the wires of the BetaCage during its assembly, an ultra-low-radon cleanroom is being commissioned at Syracuse University using a vacuum-swing-adsorption radon-mitigation system. The radon filter shows ~20$\times$ reduction at its output, from 7.47$\pm$0.56 to 0.37$\pm$0.12 Bq/m$^3$, and the cleanroom radon activity meets project requirements, with a lowest achieved value consistent with that of the filter, and levels consistently < 2 Bq/m$^3$.Comment: 5 pages, 3 figures, Proceedings of Low Radioactivity Techniques (LRT) 2013, Gran Sasso, Italy, April 10-12, 201

Real-time setup to measure radon emission during rock deformation. Implications for geochemical surveillance

Laboratory experiments can represent a valid approach to unravel the complex interplay between the geochemical behaviour of radon and rock deformation mechanisms. In light of this, we present a new real-time experimental setup for analysing in continuum the alpha-emitting 222Rn and 220Rn daughters over variable stress–strain regimes. The most innovative segment of this setup consists of the radon accumulation chamber obtained from a tough and durable material that can host large cylindrical rock samples. The accumulation chamber is connected, in a closed-loop configuration, to a gas-drying unit and to a RAD7 radon monitor. A recirculating pump moves the gas from the rock sample to a solid-state detector for alpha counting of radon and thoron progeny. The measured radon signal is enhanced by surrounding the accumulation chamber with a digitally controlled heating belt. As the temperature is increased, the number of effective collisions of radon atoms increases favouring the diffusion of radon through the material and reducing the analytical uncertainty. The accumulation chamber containing the sample is then placed into a uniaxial testing apparatus where the axial deformation is measured throughout a linear variable displacement transducer. A dedicated software allows obtaining a variety of stress–strain regimes from fast deformation rates to long-term creep tests. Experiments conducted with this new real-time setup have important ramifications for the interpretation of geochemical anomalies recorded prior to volcanic eruptions or earthquakes

Active and passive radon concentration measurements and first-step mapping in schools of Banja Luka, Republic of Srpska

Radon concentration measurements were performed in all 25 primary schools in Banja Luka city, the capital of Republika Srpska, during 2011 and 2012, using both active RAD7 continual radon measuring instruments and CR-39 passive (commercially known as Gamma) detectors. The two complimentary methods were employed not only to obtain annual averages, but also to study the dynamics of radon concentration changes during the week. For each school, average and temporal variations of radon concentrations were analysed, taking into consideration local geology, building materials and meteorological conditions. The influence of forced ventilation, caused by frequent opening of doors and windows during working hours, with typical dawn and weekend peaks is evident in most but not all schools. Elevated levels of radon concentration (>400 Bq m-3) were found in a few schools using both methods. Although high correlation factor of 0.8 between passive and active methods was found, still short-time (one-week) measurements cannot be used for annual estimation of radon activity but screening one. Thus, the conclusion concerns only long time measurements as valid indicator of annual radon activity.JRC.E.8-Nuclear securit

Demonstration of radon removal from SF6 using molecular sieves

The gas SF6 has become of interest as a negative ion drift gas for use in directional dark matter searches. However, as for other targets in such searches, it is important that radon contamination can be removed as this provides a source of unwanted background events. In this work we demonstrate for the first time filtration of radon from SF6 gas by using a molecular sieve. Four types of sieves from Sigma-Aldrich were investigated, namely 3Å, 4Å, 5Å and 13X. A manufactured radon source was used for the tests. This was attached to a closed loop system in which gas was flowed through the filters and a specially adapted Durridge RAD7 radon detector. In these measurements, it was found that only the 5Å type was able to significantly reduce the radon concentration without absorbing the SF6 gas. The sieve was able to reduce the initial radon concentration of 3875 ± 13 Bqm−3 in SF6 gas by 87% when cooled with dry ice. The ability of the cooled 5Å molecular sieve filter to significantly reduce radon concentration from SF6 provides a promising foundation for the construction of a radon filtration setup for future ultra-sensitive SF6 gas rare-event physics experiments