Neutron scattering studies of Zn-doped La2-xSrxCuO4

This paper reviews studies of the spatial modulation of spin in La2-xSrxCuO4 (LSCO) through neutron-scattering measurements of the elastic magnetic peaks, with emphasis on Zn-doped LSCO. The elastic incommensurate magnetic peaks can be categorized in two classes with respect to the temperature dependence. Nd-doped LSCO, La2CuO4+y and LSCO with x ~ 1/8 exhibit an ordinary power law behavior. On the other hand, Zn-doped LSCO and LSCO with x = 0.02-0.07 show an exponential temperature dependence, and the correlation lengths stay short. This discrepancy can be attributed to the difference in the mechanism of pinning spin fluctuations. The former systems have pinning centers which is coherent to the lattice. In the latter, however, pinning centers are randomly scattered in the CuO2 planes, thus incoherent. The incoherent pinning model is discussed with referring to recent mu-SR studies.Comment: 6 pages, including 4 figures and 1 table. Proceedings for ISS2000 (Tokyo, October 2000

Thermal Conductivity of Pr_{1.3-x}La_{0.7}Ce_xCuO_4 Single Crystals and Signatures of Stripes in an Electron-Doped Cuprate

It was recently demonstrated that the anisotropic phonon heat transport behavior is a good probe of the stripe formation in La_{2-x}Sr_xCuO_4 (LSCO) [X. F. Sun {\it et al.}, Phys. Rev. B {\bf 67}, 104503 (2003)]. Using this probe, we examined an electron-doped cuprate Pr_{1.3-x}La_{0.7}Ce_xCuO_4 (PLCCO) and found that essentially the same features as those in LSCO are observed. Moreover, the in-plane resistivity \rho_{ab} of lightly-doped PLCCO shows metallic behavior (d\rho_{ab}/dT > 0) in the N\'eel ordered state with a mobility comparable to that in LSCO. It is discussed that these peculiar properties in common with LSCO signify the existence of stripes in electron-doped cuprates.Comment: 4 pages, 4 figures, revised version accepted for publication in Phys. Rev. Let

Structural, magnetic and superconducting properties of pulsed-laser-deposition-grown La1.85Sr0.15CuO4/La2/3Ca1/3MnO3\rm{La_{1.85}Sr_{0.15}CuO_{4}/La_{2/3}Ca_{1/3}MnO_{3}} superlattices on (001)\rm{(001)}-oriented LaSrAlO4\rm{LaSrAlO_{4}} substrates

Epitaxial La1.85Sr0.15CuO4/La2/3Ca1/3MnO3 superlattices on (001)-oriented LaSrAlO4 substrates have been grown with pulsed laser deposition technique. Their structural, magnetic and superconducting properties have been determined with in-situ reflection high energy electron diffraction, x-ray diffraction, specular neutron reflectometry, scanning transmission electron microscopy, electric transport, and magnetization measurements. We find that despite the large mismatch between the in-plane lattice parameters of LSCO and LCMO these superlattices can be grown epitaxially and with a high crystalline quality. While the first LSCO layer remains clamped to the LSAO substrate, a sizeable strain relaxation occurs already in the first LCMO layer. The following LSCO and LCMO layers adopt a nearly balanced state in which the tensile and compressive strain effects yield alternating in-plane lattice parameters with an almost constant average value. No major defects are observed in the LSCO layers, while a significant number of vertical antiphase boundaries are found in the LCMO layers. The LSCO layers remain superconducting with a relatively high superconducting onset temperature of about 36 K. The macroscopic superconducting response is also evident in the magnetization data due to a weak diamagnetic signal below 10 K for H || ab and a sizeable paramagnetic shift for H || c that can be explained in terms of a vortex-pinning-induced flux compression. The LCMO layers maintain a strongly ferromagnetic state with a Curie temperature of about 190 K and a large low-temperature saturation moment of about 3.5(1) muB. These results suggest that the LSCO/LCMO superlattices can be used to study the interaction between the antagonistic ferromagnetic and superconducting orders and, in combination with previous studies on YBCO/LCMO superlattices, may allow one to identify the relevant mechanisms.Comment: 13 pages, 11 figure

Evidence for suppressed metallicity on the surface of La2-xSrxCuO4 and Nd2-xCexCuO4

Hard X-ray Photoemission spectroscopy (PES) of copper core electronic states, with a probing depth of $\sim$60 \AA, is used to show that the Zhang-Rice singlet feature is present in La$_2$CuO$_4$ but is absent in Nd$_2$CuO$_4$. Hole- and electron doping in La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) and Nd$_{2-x}$Ce$_x$CuO$_4$ (NCCO) result in new well-screened features which are missing in soft X-ray PES. Impurity Anderson model calculations establish metallic screening as its origin, which is strongly suppressed within 15 $\text{\AA}$ of the surface. Complemented with X-ray absorption spectroscopy, the small chemical-potential shift in core levels ($\sim0.2$ eV) are shown to be consistent with modifications of valence and conduction band states spanning the band gap ($\sim1$ eV) upon hole- and electron-doping in LSCO and NCCO.Comment: 4 pages, 4 figure

Thermal conductivity of lightly Sr- and Zn-doped La2_2CuO4_4 single crystals

Both ab-plane and c-axis thermal conductivities ($\kappa_{ab}$ and $\kappa_c$) of lightly doped La$_{2-x}$Sr$_x$CuO$_4$ and La$_2$Cu$_{1-y}$Zn$_y$O$_4$ single crystals ($x$ or $y$ = 0 -- 0.04) are measured from 2 to 300 K. It is found that the low-temperature phonon peak (at 20 -- 25 K) is significantly suppressed upon Sr or Zn doping even at very low doping, though its precise doping dependences show interesting differences between the Sr and Zn dopants, or between the $ab$ plane and the c axis. Most notably, the phonon peak in $\kappa_c$ decreases much more quickly with Sr doping than with Zn doping, while the phonon-peak suppression in $\kappa_{ab}$ shows an opposite trend. It is discussed that the scattering of phonons by stripes is playing an important role in the damping of the phonon heat transport in lightly doped LSCO, in which static spin stripes has been observed by neutron scattering. We also show $\kappa_{ab}$ and $\kappa_c$ data of La$_{1.28}$Nd$_{0.6}$Sr$_{0.12}$CuO$_4$ and La$_{1.68}$Eu$_{0.2}$Sr$_{0.12}$CuO$_4$ single crystals to compare with the data of the lightly doped crystals for the discussion of the role of stripes. At high temperature, the magnon peak (i.e., the peak caused by the spin heat transport near the N\'{e}el temperature) in $\kappa_{ab}(T)$ is found to be rather robust against Zn doping, while it completely disappears with only 1% of Sr doping.Comment: 7 pages, 4 figures, accepted for publication in Phys. Rev.

Oxygen phonon branches in overdoped La1.7_{1.7}Sr0.3_{0.3}CuO4_4

The dispersion of the Cu-O bond-stretching vibrations in overdoped La$_{1.7}$Sr$_{0.3}$CuO$_4$ (not superconducting) has been studied by high resolution inelastic neutron scattering. It was found that the doping-induced renormalization of the so-called breathing and the half-breathing modes is larger than in optimally doped La$_{1.85}$Sr$_{0.15}$CuO$_4$. On the other hand, the phonon linewidths are generally smaller in the overdoped sample. Features observed in optimally doped La$_{1.85}$Sr$_{0.15}$CuO$_4$ which suggest a tendency towards charge stripe formation are absent in overdoped La$_{1.7}$Sr$_{0.3}$CuO$_4$.Comment: 6 pages, 8 figure