Thermal Transport at the Nanoscale: A Fourier\u27s Law vs. Phonon Boltzmann Equation Study

Steady-state thermal transport in nanostructures with dimensions comparable to the phonon mean-free-path is examined. Both the case of contacts at different temperatures with no internal heat generation and contacts at the same temperature with internal heat generation are considered. Fourier’s Law results are compared to finite volume method solutions of the phonon Boltzmann equation in the gray approximation. When the boundary conditions are properly specified, results obtained using Fourier’s Law without modifying the bulk thermal conductivity are in essentially exact quantitative agreement with the phonon Boltzmann equation in the ballistic and diffusive limits. The errors between these two limits are examined in this paper. For the four cases examined, the error in the apparent thermal conductivity as deduced from a correct application of Fourier’s Law is less than 6%. We also find that the Fourier’s Law results presented here are nearly identical to those obtained from a widely used ballistic-diffusive approach, but analytically much simpler. Although limited to steady-state conditions with spatial variations in one dimension and to a gray model of phonon transport, the results show that Fourier’s Law can be used for linear transport from the diffusive to the ballistic limit. The results also contribute to an understanding of how heat transport at the nanoscale can be understood in terms of the conceptual framework that has been established for electron transport at the nanoscale

Fourier's Law: insight from a simple derivation

The onset of Fourier's law in a one-dimensional quantum system is addressed via a simple model of weakly coupled quantum systems in contact with thermal baths at their edges. Using analytical arguments we show that the crossover from the ballistic (invalid Fourier's law) to diffusive (valid Fourier's law) regimes is characterized by a thermal length-scale, which is directly related to the profile of the local temperature. In the same vein, dephasing is shown to give rise to a classical Fourier's law, similarly to the onset of Ohm's law in mesoscopic conductors.Comment: 4+ pages, references and discussions adde

Quantum transport efficiency and Fourier's law

We analyze the steady-state energy transfer in a chain of coupled two-level systems connecting two thermal reservoirs. Through an analytic treatment we find that the energy current is independent of the system size, hence violating Fourier's law of heat conduction. The classical diffusive behavior in Fourier's law of heat conduction can be recovered by introducing decoherence to the quantum systems constituting the chain. Implications of these results on energy transfer in biological light harvesting systems, and the role of quantum coherences and entanglement are discussed.Comment: 6 pages, 4 figure

Reconstructing Fourier's law from disorder in quantum wires

The theory of open quantum systems is used to study the local temperature and heat currents in metallic nanowires connected to leads at different temperatures. We show that for ballistic wires the local temperature is almost uniform along the wire and Fourier's law is invalid. By gradually increasing disorder, a uniform temperature gradient ensues inside the wire and the thermal current linearly relates to this local temperature gradient, in agreement with Fourier's law. Finally, we demonstrate that while disorder is responsible for the onset of Fourier's law, the non-equilibrium energy distribution function is determined solely by the heat baths