Early onset of ground-state deformation in the neutron-deficient polonium isotopes

In-source resonant ionization laser spectroscopy of the even-$A$ polonium isotopes $^{192-210,216,218}$Po has been performed using the $6p^37s$ $^5S_2$ to $6p^37p$ $^5P_2$ ($\lambda=843.38$ nm) transition in the polonium atom (Po-I) at the CERN ISOLDE facility. The comparison of the measured isotope shifts in $^{200-210}$Po with a previous data set allows to test for the first time recent large-scale atomic calculations that are essential to extract the changes in the mean-square charge radius of the atomic nucleus. When going to lighter masses, a surprisingly large and early departure from sphericity is observed, which is only partly reproduced by Beyond Mean Field calculations.Comment: As submitted to PR

Why is lead so kinky?

We revisit the problem of the kink in the charge radius shift of neutron-rich even lead isotopes. We show that the ability of a Skyrme force to reproduce the isotope shift is determined by the occupation of the neutron 1i11/2 orbital beyond N=126 and the corresponding change it causes to deeply-bound protons orbitals with a principal quantum number of 1. Given the observed position of the single-particle energies, one must either ensure occupation is allowed through correlations, or not demand that the single-particle energies agree with experimental values at the mean-field level.Comment: 5 pages, 5 figure

Nuclear shape coexistence in Po isotopes: An interacting boson model study

Background: The lead region, Po, Pb, Hg, and Pt, shows up the presence of coexisting structures having different deformation and corresponding to different particle-hole configurations in the Shell Model language. Purpose: We intend to study the importance of configuration mixing in the understanding of the nuclear structure of even-even Po isotopes, where the shape coexistence phenomena are not clear enough. Method: We study in detail a long chain of polonium isotopes, 190-208Po, using the interacting boson model with configuration mixing (IBM-CM). We fix the parameters of the Hamiltonians through a least-squares fit to the known energies and absolute B(E2) transition rates of states up to 3 MeV. Results: We obtained the IBM-CM Hamiltonians and we calculate excitation energies, B(E2)'s, electric quadrupole moments, nuclear radii and isotopic shifts, quadrupole shape invariants, wave functions, and deformations. Conclusions: We obtain a good agreement with the experimental data for all the studied observables and we conclude that shape coexistence phenomenon is hidden in Po isotopes, very much as in the case of the Pt isotopes.Comment: To be published in Physical Review C. arXiv admin note: text overlap with arXiv:1312.459

Unique and complementary information on shape coexistence in the neutron-deficient Pb region derived from Coulomb excitation

Neutron-deficient isotopes of Pt–Hg–Pb–Po–Rn are the classic region in the investigation of shape coexistence in atomic nuclei. A large programme of Coulomb-excitation experiments has been undertaken at the REX-ISOLDE facility in CERN with a number of even–even isotopes in this region. These experiments have been used to probe the electromagnetic properties of yrast and non-yrast states of even–even exotic nuclei, above and below Z = 82. Amongst a large amount of different complementary techniques used to study nuclear structure, Coulomb excitation brings substantial and unique information detailing shape coexistence. In this paper we review the Coulomb-excitation campaign at REX-ISOLDE in the light-lead region together with most recently obtained results. Furthermore, we present some new interpretations that arise from this data and show testing comparisons to state-of-the-art nuclear models

Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes

Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po-196,Po-198,Po-200,Po-202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po-196,Po-198, the transitional and diagonal matrix elements of the 2(1)(+) state are determined. In Po-196,Po-198 multistep Coulomb excitation is observed, populating the 4(1)(+), 0(2)(+), and 2(2)(+) states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po-196 onwards. Three model descriptions are used to compare to the data. Calculations with the beyond-mean-field model, the interacting boson model, and the general Bohr Hamiltonian model show partial agreement with the experimental data. Finally, calculations with a phenomenological two-level mixing model hint at the mixing of a spherical structure with a weakly deformed rotational structure.Peer reviewe

Systematic shell-model study for structure and isomeric states in 200−210^{200-210}Po isotopes

We report systematic large-scale shell-model calculation for Po isotopes with $A=$ 200 to 210. We have performed calculations using KHH7B interaction in the model space $Z$ = 58-114 and $N$ = 100-164 around doubly-magic $^{208}$Pb. We allow valence neutrons to occupy in the $1f_{5/2}$, $2p_{3/2}$, $2p_{1/2}$, and $0i_{13/2}$ orbitals, while two valence protons beyond $Z=82$ are occupied in $0h_{9/2}$, $1f_{7/2}$ and $0i_{13/2}$ orbitals. The calculated energies and electromagnetic properties are compared with the available experimental data and predicted where experimental data are not available. We have also reported shell-model results for different isomeric states of these nuclei.Comment: 20 pages, 11 figure