We apply the microscopic coupled-cluster method (CCM) to the spin-21XXZ models on both the one-dimensional chain and the two-dimensional square
lattice. Based on a systematic approximation scheme of the CCM developed by us
previously, we carry out high-order {\it ab initio} calculations using
computer-algebraic techniques. The ground-state properties of the models are
obtained with high accuracy as functions of the anisotropy parameter.
Furthermore, our CCM analysis enables us to study their quantum critical
behavior in a systematic and unbiased manner.Comment: (to appear in PRL). 4 pages, ReVTeX, two figures available upon
request. UMIST Preprint MA-000-000