We report on the Fe17 high-spin molecular cluster and show that this system
is an exemplification of nanostructured dipolar magnetism. Each Fe17 molecule,
with spin S=35/2 and axial anisotropy as small as D=-0.02K, is the magnetic
unit that can be chemically arranged in different packing crystals whilst
preserving both spin ground-state and anisotropy. For every configuration,
molecular spins are correlated only by dipolar interactions. The ensuing
interplay between dipolar energy and anisotropy gives rise to macroscopic
behaviors ranging from superparamagnetism to long-range magnetic order at
temperatures below 1K.Comment: Replaced with version accepted for publication in Physical Review
Letter