Although most known non-Fermi liquid (NFL) materials are structurally or
chemically disordered, the role of this disorder remains unclear. In
particular, very few systems have been discovered that may be stoichiometric
and well ordered. To test whether U3Ni3Sn4 belongs in this latter class, we
present measurements of the x-ray absorption fine structure (XAFS) of
polycrystalline and single-crystal U3Ni3Sn4 samples that are consistent with no
measurable local structural disorder. We also present temperature-dependent
specific heat data in applied magnetic fields as high as 8 T that show features
that are inconsistent with the antiferromagnetic Griffiths' phase model, but do
support the conclusion that a Fermi liquid/NFL crossover temperature increases
with applied field. These results are inconsistent with theoretical
explanations that require strong disorder effects, but do support the view that
U3Ni3Sn4 is a stoichiometric, ordered material that exhibits NFL behavior, and
is best described as being near an antiferromagnetic quantum critical point.Comment: 9 pages, 8 figures, in press with PR
