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Schwinger-Boson Mean-Field Theory of Mixed-Spin Antiferromagnet L2BaNiO5L_2BaNiO_5

Abstract

The Schwinger-boson mean-field theory is used to study the three-dimensional antiferromagnetic ordering and excitations in compounds L2BaNiO5L_2BaNiO_5, a large family of quasi-one-dimensional mixed-spin antiferromagnet. To investigate magnetic properties of these compounds, we introduce a three-dimensional mixed-spin antiferromagnetic Heisenberg model based on experimental results for the crystal structure of L2BaNiO5L_2BaNiO_5. This model can explain the experimental discovery of coexistence of Haldane gap and antiferromagnetic long-range order below N\'{e}el temperature. Properties such as the low-lying excitations, magnetizations of NiNi and rare-earth ions, N\'{e}el temperatures of different compounds, and the behavior of Haldane gap below the N\'{e}el temperature are investigated within this model, and the results are in good agreement with neutron scattering experiments.Comment: 12 pages, 6 figure

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    Last time updated on 03/01/2020