Specific heat and magnetization measurements have been performed on
high-quality single crystals of filled-skutterudite PrFe_4P_{12} in order to
study the high-field heavy-fermion state (HFS) and low-field ordered state
(ODS). From a broad hump observed in C/T vs T in HFS for magnetic fields
applied along the direction, the Kondo temperature of ~ 9 K and the
existence of ferromagnetic Pr-Pr interactions are deduced. The {141}-Pr nuclear
Schottky contribution, which works as a highly-sensitive on-site probe for the
Pr magnetic moment, sets an upper bound for the ordered moment as ~ 0.03
\mu_B/Pr-ion. This fact strongly indicates that the primary order parameter in
the ODS is nonmagnetic and most probably of quadrupolar origin, combined with
other experimental facts. Significantly suppressed heavy-fermion behavior in
the ODS suggests a possibility that the quadrupolar degrees of freedom is
essential for the heavy quasiparticle band formation in the HFS. Possible
crystalline-electric-field level schemes estimated from the anisotropy in the
magnetization are consistent with this conjecture.Comment: 7 pages and 7 figures. Accepted for publication in Phys. Rev.