Applying machine learning methods for characterization of hexagonal prisms from their 2D scattering patterns – an investigation using modelled scattering data

Abstract

This document is the Accepted Manuscript version of the following article: Emmanuel Oluwatobi Salawu, Evelyn Hesse, Chris Stopford, Neil Davey, and Yi Sun, 'Applying machine learning methods for characterization of hexagonal prisms from their 2D scattering patterns – an investigation using modelled scattering data', Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 201, pp. 115-127, first published online 5 July 2017. Under embargo. Embargo end date: 5 July 2019. The Version of Record is available online at doi: https://doi.org/10.1016/j.jqsrt.2017.07.001. © 2017 Elsevier Ltd. All rights reserved.Better understanding and characterization of cloud particles, whose properties and distributions affect climate and weather, are essential for the understanding of present climate and climate change. Since imaging cloud probes have limitations of optical resolution, especially for small particles (with diameter < 25 μm), instruments like the Small Ice Detector (SID) probes, which capture high-resolution spatial light scattering patterns from individual particles down to 1 μm in size, have been developed. In this work, we have proposed a method using Machine Learning techniques to estimate simulated particles’ orientation-averaged projected sizes (PAD) and aspect ratio from their 2D scattering patterns. The two-dimensional light scattering patterns (2DLSP) of hexagonal prisms are computed using the Ray Tracing with Diffraction on Facets (RTDF) model. The 2DLSP cover the same angular range as the SID probes. We generated 2DLSP for 162 hexagonal prisms at 133 orientations for each. In a first step, the 2DLSP were transformed into rotation-invariant Zernike moments (ZMs), which are particularly suitable for analyses of pattern symmetry. Then we used ZMs, summed intensities, and root mean square contrast as inputs to the advanced Machine Learning methods. We created one random forests classifier for predicting prism orientation, 133 orientation-specific (OS) support vector classification models for predicting the prism aspect-ratios, 133 OS support vector regression models for estimating prism sizes, and another 133 OS Support Vector Regression (SVR) models for estimating the size PADs. We have achieved a high accuracy of 0.99 in predicting prism aspect ratios, and a low value of normalized mean square error of 0.004 for estimating the particle’s size and size PADs.Peer reviewe