The laser-like coherent emission at 391nm from N2​ gas irradiated by strong
800nm pump laser and weak 400nm seed laser is theoretically investigated.
Recent experimental observations are well simulated, including temporal
profile, optical gain and periodic modulation of the 391nm signal from N2+​.
Our calculation sheds light on the long standing controversy on whether
population inversion is indispensable for the optical gain. We demonstrate the
Ramsey interference fringes of the emission intensity at 391nm formed by
additionally injecting another 800nm pump or 400nm seed, which are well
explained by the coherent modulation of transition dipole moment and population
between the A2Πu​(ν=2)-X2Σg+​ states as well as the
B2Σu+​(ν=0)-X2Σg+​ states. This study provides versatile
possibilities for the coherent control of N2+​ air laser.Comment: 5 pages, 5 figure