We have conducted a spectroscopic survey of 78 starbursting infrared-luminous
galaxies at redshifts up to z = 0.5. We use moderate-resolution spectroscopy of
the NaI D interstellar absorption feature to directly probe the neutral phase
of outflowing gas in these galaxies. Over half of our sample are ultraluminous
infrared galaxies that are classified as starbursts; the rest have infrared
luminosities in the range log(L_IR/L_sun) = 10.2 - 12.0. The sample selection,
observations, and data reduction are described here. The absorption-line
spectra of each galaxy are presented. We also discuss the theory behind
absorption-line fitting in the case of a partially-covered, blended absorption
doublet observed at moderate-to-high resolution, a topic neglected in the
literature. A detailed analysis of these data is presented in a companion
paper.Comment: 59 pages, 18 figures in AASTeX preprint style; to appear in September
issue of ApJ