Single photon sources (SPSs) based on quantum emitters hold promise in
quantum radiometry as metrology standard for photon fluxes at the low light
level. Ideally this requires control over the photon flux in a wide dynamic
range, sub-Poissonian photon statistics and narrow-band emission spectrum. In
this work, a monochromatic single-photon source based on an organic dye
molecule is presented, whose photon flux is traceably measured to be adjustable
between 144 000 and 1320 000 photons per second at a wavelength of (785.6 +/-
0.1) nm, corresponding to an optical radiant flux between 36.5 fW and 334 fW.
The high purity of the single-photon stream is verified, with a second-order
autocorrelation function at zero time delay below 0.1 throughout the whole
range. Featuring an appropriate combination of emission properties, the
molecular SPS shows here application in the calibration of a silicon
Single-Photon Avalanche Detector (SPAD) against a low-noise analog silicon
photodiode traceable to the primary standard for optical radiant flux (i.e. the
cryogenic radiometer). Due to the narrow bandwidth of the source, corrections
to the SPAD detection efficiency arising from the spectral power distribution
are negligible. With this major advantage, the developed device may finally
realize a low-photon-flux standard source for quantum radiometry