We report experimental demonstration of continuous-wave cascaded-harmonic
generation and Raman lasing in a millimeter-scale lithium niobate
whispering-gallery resonator pumped at a telecommunication-compatible infrared
wavelength. Intensity enhancement through multiple recirculations in the
whispering-gallery resonator and quasi phase-matching through a nonuniform
crystal poling enable simultaneous cascaded-harmonic generation up to the
fourth-harmonic accompanied by stimulated Raman, two-photon, three-photon, and
four-photon Raman scattering corresponding the molecular vibrational
wavenumbers 632 cm-1 and 255 cm-1 in z-cut lithium niobate at pump power levels
as low as 200mW. We demonstrate simultaneous cascaded-harmonic generation and
Raman lasing by observing the spectrum of the scattered light from the
resonator and by capturing the image of the decoupled light from the resonator
on a color CCD camera
