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Charge dynamics of the Co-doped BaFe2_2As2_2

Abstract

We report on a thorough optical investigation over a broad spectral range and as a function of temperature of the charge dynamics in Ba(Cox_xFe1x_{1-x})2_2As2_2 compounds for Co-doping ranging between 0 and 18%. For the parent compound as well as for xx=0.025 we observe the opening of a pseudogap, due to the spin-density-wave phase transition and inducing a reshuffling of spectral weight from low to high frequencies. For compounds with 0.051x\le x \le 0.11 we detect the superconducting gap, while at xx=0.18 the material stays metallic at all temperatures. We describe the effective metallic contribution to the optical conductivity with two Drude terms, representing the combination of a coherent and incoherent component, and extract the respective scattering rates. We establish that the dcdc transport properties in the normal phase are dominated by the coherent Drude term for 0x\le x \le0.051 and by the incoherent one for 0.061x\le x \le0.18, respectively. Finally through spectral weight arguments, we give clear-cut evidence for moderate electronic correlations for 0x\le x \le0.061, which then crossover to values appropriate for a regime of weak interacting and nearly-free electron metals for xx\ge0.11

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