Terrace remnants of late Pleistocene fine-grained valley-fills, at present eroded by ephemeral traction-load streams, are reported from many semi-arid and arid parts of the world. While they present promising palaeo-environmental archives for recent geological times such as the Last Glacial Maximum (LGM) for which few other terrestrial depositional records exist, their poorly understood nature has limited their significance. This study examines the fine-grained valley-fill deposits from the Flinders Ranges in South Australia, here called Flinders Silts. It establishes the timing, mode and environmental controls of deposition as opposed to their advancing erosion under the current climate. A regional chronostratigraphy based on 124 numerical dates is discussed, of which 43 radiocarbon and 22 luminescence ages were obtained from 12 sections across three major catchments within the scope of this thesis. Regionally significant intervals of rapid aggradation, relative surface stability and erosion are established. Regional climatic controls are differentiated from intrinsic catchment- and site-specific effects on the system. Further, individual age proxies and age models are critically assessed in how far they reflect depositional events. The final aggradational interval bracketing the extended LGM is discussed in detail on a continuous layered to laminated stratigraphic sequence. The provenance question of the fine-grained sediments and the depositional environment of the Flinders Silts are further addressed by high-resolution particle-size analysis. In order to study the subtle variations within the fine-grained partially-aggregated material, an original parametric sediment-sizing approach is employed. Finally, a range of traditional and emerging analytical techniques are applied to improve our understanding of palaeo-environments promoting aggradation. In conclusion, arid intervals throughout the last glacial cycle resulted in significant quantities of proximal dust being deposited as loess mantles within the catchments of the Flinders Ranges, acting as a near-longitudinal dust trap in the centre of the late Pleistocene “dust bowl”. The fine-grained aeolian accessions were repeatedly eroded by low-frequency high-magnitude precipitation events and redistributed as loess-derived alluvium, congesting narrow gorges and raising the base level for tributaries. Locally, backflooding resulted in the aggradation of layered to laminated slackwater deposits, the most continuous recording at least 12 large and numerous smaller flood events between 24 ka and 18 ka. The synchronous termination of the Flinders Silts coincides with early Deglacial climatic amelioration. The re-establishment of a perennial plant cover stabilising both dune fields and slope mantes is discussed as a potential scenario that would have discontinued dust supply to the fluvial system, in turn promoting incision and erosion. The studied aeolian-fluvial interplay of loess and floods has large implications for our understanding of landscape evolution in semi-arid Australia.Thesis (Ph.D.) -- University of Adelaide, School of Earth and Environmental Sciences, 200