This work demonstrates dramatically modified spin dynamics of magnetic
insulator (MI) by the spin-momentum locked Dirac surface states of the adjacent
topological insulator (TI) which can be harnessed for spintronic applications.
As the Bi-concentration x is systematically tuned in 5 nm thick (BixSb1-x)2Te3
TI film, the weight of the surface relative to bulk states peaks at x = 0.32
when the chemical potential approaches the Dirac point. At this concentration,
the Gilbert damping constant of the precessing magnetization in 10 nm thick
Y3Fe5O12 MI film in the MI/TI heterostructures is enhanced by an order of
magnitude, the largest among all concentrations. In addition, the MI acquires
additional strong magnetic anisotropy that favors the in-plane orientation with
similar Bi-concentration dependence. These extraordinary effects of the Dirac
surface states distinguish TI from other materials such as heavy metals in
modulating spin dynamics of the neighboring magnetic layer
