Synthesis of Nitrogen-Doped
MnO/Graphene Nanosheets
Hybrid Material for Lithium Ion Batteries
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Abstract
Nitrogen-doped MnO/graphene nanosheets (N-MnO/GNS) hybrid
material
was synthesized by a simple hydrothermal method followed by ammonia
annealing. The samples were systematically investigated by X-ray diffraction
analysis, Raman spectroscopy, X-ray photoelectron spectroscopy, transmission
electron microscopy, and atomic force microscopy. N-doped MnO (N-MnO)
nanoparticles were homogenously anchored on the thin layers of N-doped
GNS (N-GNS) to form an efficient electronic/ionic mixed conducting
network. This nanostructured hybrid exhibited a reversible electrochemical
lithium storage capacity as high as 772 mAh g<sup>–1</sup> at
100 mA g<sup>–1</sup> after 90 cycles, and an excellent rate
capability of 202 mA h g<sup>–1</sup> at a high current density
of 5 A g<sup>–1</sup>. It is expected that N-MnO/GNS hybrid
could be a promising candidate material as a high capacity anode for
lithium ion batteries