Room-Temperature Negative Capacitance in a Ferroelectric–Dielectric Superlattice Heterostructure

Abstract

We demonstrate room-temperature negative capacitance in a ferroelectric–dielectric superlattice heterostructure. In epitaxially grown superlattice of ferroelectric BSTO (Ba<sub>0.8</sub>Sr<sub>0.2</sub>TiO<sub>3</sub>) and dielectric LAO (LaAlO<sub>3</sub>), capacitance was found to be larger compared to the constituent LAO (dielectric) capacitance. This enhancement of capacitance in a series combination of two capacitors indicates that the ferroelectric was stabilized in a state of negative capacitance. Negative capacitance was observed for superlattices grown on three different substrates (SrTiO<sub>3</sub> (001), DyScO<sub>3</sub> (110), and GdScO<sub>3</sub> (110)) covering a large range of substrate strain. This demonstrates the robustness of the effect as well as potential for controlling the negative capacitance effect using epitaxial strain. Room-temperature demonstration of negative capacitance is an important step toward lowering the subthreshold swing in a transistor below the intrinsic thermodynamic limit of 60 mV/decade and thereby improving energy efficiency

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