Atomically thin photodetectors based
on 2D materials have attracted great interest due to their potential
as highly energy-efficient integrated devices. However, photoinduced
carrier generation in these media is relatively poor due to low optical
absorption, limiting device performance. Current methods for overcoming
this problem, such as reducing contact resistances or back gating,
tend to increase dark current and suffer slow response times. Here,
we realize the avalanche effect in a 2D material-based photodetector
and show that avalanche multiplication can greatly enhance the device
response of an ultrathin InSe-based photodetector. This is achieved
by exploiting the large Schottky barrier formed between InSe and Al
electrodes, enabling the application of a large bias voltage. Plasmonic
enhancement of the photosensitivity, achieved by patterning arrays
of Al nanodisks onto the InSe layer, further improves device efficiency.
With an external quantum efficiency approaching 866%, a dark current
in the picoamp range, and a fast response time of 87 μs, this
atomic layer device exhibits multiple significant advances in overall
performance for this class of devices