Study of Temporal Variations of Equivalent Black Carbon in a Coastal City in Northwest Spain Using an Atmospheric Aerosol Data Management Software

Abstract

[Abstract] Light-absorbing carbonaceous aerosols (including black carbon (BC)) pose serious health issues and play significant roles in atmospheric radiative properties. Two-year measurements (2015–2016) of aerosol light absorption, combined with measurements of sub-micrometric particles, were continuously conducted in A Coruña (northwest (NW) Spain) to determine their light absorption properties: absorption coefficients (σabs) and the absorption Ångström exponent (AAE). The mean and standard deviation of equivalent black carbon (eBC) during the period of study were 0.85 ± 0.83 µg m−3, which are lower than other values measured in urban areas of Spain and Europe. High eBC concentrations found in winter are associated with an increase in emissions from anthropogenic sources in combination with lower mixing layer heights and frequent stagnant conditions. The pronounced diurnal variability suggests a strong influence from local sources. AAE had an average value of 1.26 ± 0.22 which implies that both fossil fuel combustion and biomass burning influenced optical aerosol properties. This also highlights biomass combustion in suburban areas, where the use of wood for domestic heating is encouraged, as an important source of eBC. All data treatment was gathered using SCALA© as atmospheric aerosol data management support software program.This research was funded by the Spanish R&D Plan (PROACLIM project: CGL2014-52877-R and CRISOL project: CGL2017-85344-R) and by the Xunta de Galicia (GRC2013-047 and ED431C 2017/28).Xunta de Galicia; GRC2013-047Xunta de Galicia; ED431C 2017/2