The shift due to Jovian gravitational deflection in the apparent angular position of the radio source P 0201+113 was measured with very long baseline interferometry (VLBI) to demonstrate a differential angular tracking technique with nanoradian accuracy. The raypath of the radio source P 0201+113 passed within 1 mrad of Jupiter (approximately 10 Jovian radii) on 21 Mar. 1988. Its angular position was measured 10 times over 4 hours on that date, with a similar measurement set on 2 Apr. 1988, to track the differential angular gravitational deflection of the raypath. According to general relativity, the expected gravitational bend of the raypath averaged over the duration of the March experiment was approximately 1.45 nrad projected onto the two California-Australia baselines over which it was measured. Measurement accuracies on the order of 0.78 nrad were obtained for each of the ten differential measurements. The chi(exp 2) per degree of freedom of the data for the hypothesis of general relativity was 0.6, which suggests that the modeled dominant errors due to system noise and tropospheric fluctuations fully accounted for the scatter in the measured angular deflections. The chi(exp 2) per degree of freedom for the hypothesis of no gravitational deflection by Jupiter was 4.1, which rejects the no-deflection hypothesis with greater than 99.999 percent confidence. The system noise contributed about 0.34 nrad per combined-baseline differential measurement and tropospheric fluctuations contributed about 0.70 nrad. Unmodeled errors were assessed, which could potentially increase the 0.78 nrad error by about 8 percent. The above chi(exp 2) values, which result from the full accounting of errors, suggest that the nanoradian gravitational deflection signature was successfully tracked