Berges, B.J.P.

Leighton, T.G.

Tomczk, M.

White, P.R.

Wright, I.C.

English

NERC Open Research Archive

Proceedings of the 11th European Conference on Underwater Acoustics ACOUSTIC DETECTION OF SEABED GAS LEAKS, WITH APPLICATION TO CARBON CAPTURE AND STORAGE (CCS), AND LEAK PREVENTION FOR THE OIL AND GAS INDUSTRY: PRELIMINARY ASSESSMENT OF USE OF ACTIVE AND PASSIVE ACOUSTIC INVERSION FOR THE QUANTIFICATION OF UNDERWATER GAS RELEASES  B. J. P. Bergès Institute of Sound and Vibration Research, University of Southampton, UK  T. G. Leighton Institute of Sound and Vibration Research, University of Southampton, UK P. R. White Institute of Sound and Vibration Research, University of Southampton, UK M. Tomczyk University of Bremen, Marum, Bremen, Germany I.C. Wright National Oceanography Center, Southampton, United Kingdom  1 INTRODUCTION The acoustic remote sensing of subsea gas leakage is becoming increasingly important. This includes the monitoring of underwater discharges from human related and natural sources, for the following reasons. First, as the oil and gas industry faces increasing regulation from authorities, there is a need to put more control in the industrial process and to assess the impact of activities on the marine environment [1]. The applications are diverse, including: early warnings of “blow-out” from offshore installations, detection of leaks from underwater gas pipelines, gas leakage detection from Carbon and Capture and Storage facilities (a process aimed at mitigating the release of large quantities of     in the atmosphere), and seabed monitoring (for the stability of civil engineering project and prediction of underwater landslip) [1,2]. Second, this technology has a role to play in oceanography for a better understanding of natural occurrences of gas release from the seafloor such as gas seepage or mud volcanoes. This is of major importance for the assessment of the exchange of gas between the ocean and the atmosphere with application to global warming. All those phenomena involved the formation and release of bubbles of different sizes (from tiny bubble streams to large bubble clouds). These can be detected acoustically (using passive and active acoustic techniques) because they are strong sources and scatterers of sound [3,4].  This paper reports progress to date on an ongoing two-phase study. This project is aimed at assessing the accuracy of active and passive acoustic techniques for the quantification of gas releases with application to methane seepage and gas leaks from pipelines.  First, water tank experiments consisting of the release of clouds of bubbles were undertaken in order to estimate acoustically the bubble generation rates and correlate the results with independent measurement of flow rates. The acoustic emissions are monitored using calibrated hydrophones and post processed signals are used to infer the bubble populations using the model derived by Leighton and White [5]. The results are compared to assess the application and the accuracy of the technique.  Second, a multifrequency inversion model of single beam echosounder data from bubbles is proposed. This model is applied to EK60 data collected during the JCR253 scientific cruise [6] that observed bubble plumes formed from methane seepage venting from the seabed of the West Spitsbergen continental margin.  2 PASSIVE ACOUSTIC INVERSION 146Proceedings of the 11th European Conference on Underwater Acoustics   2.1 Procedure Measurements of passive acoustic emissions of bubble clouds were conducted in an 8 m x 8 m x 5 m deep test tank containing fresh water at 10°C. The bubble generation system used consisted on an arrangement of needles in circle on a plate. The spacing between them was approximately 3 cm and the size of each nozzle was 1.2 mm. A nitrogen gas cylinder was used to produce the gas for generating the bubbles. The output of the bottle was connected to a mass flow meter (Bronkhorst in-flow series, model F-111BI) adjusting the gas flow. The measurements of gas flow were recorded via a data acquisition system (DAQ). The bubble generation system was then connected to the end of the gas line and deployed at the bottom of the test tank.  For the acquisition of the acoustic signals, a calibrated T8105 B&K hydrophone was placed at a range of 5 meters from the base of the bubble cloud. This was connected to a B&K T2635 charge amplifier and a data acquisition unit.   Figure 1: schematic of the experimental apparatus. Bubbles were released using a nitrogen gas bottle and a bubbling system composed of six needles. The acoustic emissions were recording using a calibrated hydrophone and the flow rate was acquired using a mass flow meter connected to independent acquisition units.  The recorded signals were bandpass filtered and corrected to account for the reverberation of the enclosure. This correction is based on the theory by Cochard et al. [7] that expresses the emission in free field from given measurements in a reverberant environment. For this experiment, the volume of the test tank is         and the reverberation time is          .  From the data collected by the hydrophone, the bubble size distributions are determined using the model by Leighton and White [5]. The power spectral density  ( ) of the signal can be expressed as:      ( )   ∫  (  )|  (    )|         (1)  147Proceedings of the 11th European Conference on Underwater Acoustics    with |  (    )|  denoting the squared magnitude of the Fourier transform of the response of a single bubble of radius   . The quantity  (  ) is the bubble-emission size distribution as a function of   , defined such that ∫  (  )        represents the number of bubbles generated per second with a radius in the range (     ).   This problem can be solved numerically as the equation defines a Fredholm integral of the first kind that can be discretized [5]. The determination of the bubble distributions consists on solving the inverse problem expressed in matrix form as:             (2)   The number of radius bins is chosen to be equal to the number of frequency bins in order to build a square problem. However, the problem remains ill-posed which means that the inevitable measurement errors in  ( ) are magnified. Tikhonov regularisation is applied in order to achieve a positive and stable solution for (  ). Assuming spherical bubbles, the flow rate is calculated as follows:           ∫  (  )           (3)   This gives the final results that are compared to the independent measures from the mass flow meter (suitable corrections being made for the hydrostatic pressure imparted by the ~5 m of water). The comparison is made for nine flow rate regimes covering more than an order of magnitude in gas flow rate.  2.2 Results  Figure 2: Comparison of different flow rates calculated at different regimes and plotted in a log scale. The values represented by the red curve with stars are the measurements from the mass flow meter. The black dotted line with squares is the flow rates inferred from the acoustic signal 148Proceedings of the 11th European Conference on Underwater Acoustics   generated by the needles system. The error bars represent the uncertainty resulting from the background noise of the recordings which represents                when inverted.  The gas flow rates calculated using the inversion process described in the previous section is compared to measurements from the mass flow meter. The results for the nine regimes are shown in figure 2. Error bars show the uncertainty on the bubble count arising from the background noise. From this plot, it is noticeable that there is a good agreement at the highest flow rates. However, as the gas flux becomes smaller, the background noise contribution becomes increasingly significant compared to the bubble signal and so the difference with the mass flow meter measures becomes greater. The level calculated from the acoustic signals stabilizes when the flow rate becomes low (regimes 6-9) where the measurements are dominated by noise.  The model studied in this paper aim to quantify gas fluxes for large gas release events. However, for small events as observed by Leifer and Tang [8], presenting low flow rate, the model might not be appropriate because when individual bubble signatures can be identified, the time between these signatures contains just noise and as these intervals become longer, noise increasingly contributes to the spectrum. Identification of bubble generate rates in the natural world dates from the 1980s, and has been applied to waterfalls [9], ocean wave breaking [10], and rainfall over the ocean [11,12] and, more recently, explored to examine to bubble emissions from seeps [8, 13,14]. A combination of the two techniques possibly offers a good cover of flow rate ranges.    3 ACTIVE ACOUSTIC INVERSION During JR253 cruise on August 2011 to the West Spitsbergen region, areas that exhibited strong methane venting during JR211 cruise [15] were investigated. In addition new gas plumes have been discovered in shallow depth regions (range of 80-100 m). The acoustic surveys were conducted using an EK60 single beam multifrequency echosounder scanning at three frequencies: 38 kHz, 120 kHz and 200 kHz. As the EK60 is a calibrated system, scattering cross-section per unit volume    could be calculated from the raw data and an example is show in figure 3. The echograms at three frequencies are presented and strong bubble plumes escaping from the seafloor can be observed at 5 minutes time. In this study, those echo levels are used to infer bubble abundances using an inversion technique based on the study by Vagle and Farmer [16], similar to methods used in fisheries acoustics for the calculation of fish densities [17].   Depending on the frequency, a gas bubble is responding differently to an acoustic field. More specifically, the scattering behaviour of an object can be described by it scattering cross section    . In the specific case of a spherical gas bubble, the theory was recently reviewed by Ainslie and Leighton [18] and is used for the calculation of    in this study. The difference of echo level at different frequencies is directly related to the density of bubbles of different sizes and is used to calculate bubble abundances. At a frequency   , the backscattering volume expressed as inverse meter (   ) is related to the bubble distribution as followed:         ∫   (     )  (  )       (4)   with  (  ) the bubble size distribution expressed in number of bubbles per cubic meters. This equation defines a Fredholm integral of the first kind that can be discretized. The determination of  (  ) consists on solving the following inverse problem expressed in matrix form:              (5)   149Proceedings of the 11th European Conference on Underwater Acoustics   Using the data collected by the EK60, inversion is performed using backscattering volume levels from the bubble plumes at different frequencies from data set as presented in figure 3. The number of radius bins is chosen to be equal to the number of frequency bins in order to build a square problem. This problem also tends to be ill-posed because of inevitable errors in    and Tikhonov regularization is applied to control the growth of errors. The result of using such an approach will be a bubble size distribution based on the bubble in three frequency bins only, as the EK60 system gives echo levels at 38 kHz, 120 kHz and 200 kHz. Algorithms such as the one described by Lebourges-Dhaussy [19] that is used for zooplankton classification seem to be well suited for solving the problem stated in this study with increased number of radius bins while having a low number of frequency bins. a)  b)  150Proceedings of the 11th European Conference on Underwater Acoustics   c)   Figure 3: this figure shows echograms from data collected during JCR253 scientific cruise using the EK60 single beam multifrequency echosounder. From the top to the bottom, the frequencies are a) 38 kHz, b) 120 kHz, c) 200 kHz. The scattering cross-sections per unit volume    are plotted versus time (minutes) and depth (meter). Strong bubble plumes can be observed, starting at 5 minutes time.    4 CONCLUSION Active and passive acoustic measurements were performed and presented in this paper. First, the accuracy of a passive acoustic inversion model for the quantification of high flow rate gas leaks proposed by Leighton and White [5] was studied. Comparisons were made between measures from a calibrated hydrophone and a mass flow meter. Second, a three point inversion technique is presented with data it can be applied to.  ACKNOWLEDGEMENTS The studentship of Mr Bergès is sponsored by Statoil Ltd. The studentship of Mr. Tomczyk is sponsored by the SENSEnet project within an EU Framework 7 funded Marie Curie Initial Training Network. The data from the JCR253 scientific cruise presented in this report belong to the National Oceanography Centre, Southampton, UK. The authors thank Dr Trond Erland Bustnes of Statoil for providing guidance on industrial practicalities and requirements.  REFERENCES   1. Chris, T., Subsea leak detection. Exploration & Production, 2007. 6(1). 2. Leighton, T.G.,  Theory for acoustic propagation in marine sediment containing gas bubbles which may pulsate in a non-stationary nonlinear manner, Geophysical Research Letters, 2007. 34: L17607 3. Leighton, T.G., The acoustic bubble1994, London: Academic Press. xxvi, 613 p. 4. Ainslie, M.A. and Leighton, T.G. Near resonant bubble acoustic cross-section corrections, including examples from oceanography, volcanology, and biomedical ultrasound, Journal of the Acoustical Society of America, 2009. 126(5): p. 2163-2175. 5. Leighton, T.G. and P.R. White, Quantification of undersea gas leaks from carbon capture and storage facilities, from pipelines and from methane seeps, by their acoustic emissions. 151Proceedings of the 11th European Conference on Underwater Acoustics   Proceedings of the Royal Society a-Mathematical Physical and Engineering Sciences, 2012. 468(2138): p. 485-510. 6.  JR253 cruise plan. Lastly visited: 30/04/2012 http://www.antarctica.ac.uk/documents/cruise/JCR253%20Cruise%20Plan_compressed.pdf 7.  Cochard, N., J.L. Lacoume, P. Arzelies, and Y. Gabillet, Underwater acoustic noise measurement in test tanks. Ieee Journal of Oceanic Engineering, 2000. 25(4): p. 516-522. 8. Leifer, I. and D.J. Tang, The acoustic signature of marine seep bubbles. Journal of the Acoustical Society of America, 2007. 121(1): p. El35-El40. 9.  Leighton, T. G. and Walton, A. J. An experimental study of the sound emitted from gas bubbles in a liquid. Eur. J. Phys.  1987. 8: p. 98–104. (doi:10.1088/0143-0807/8/2/005) 10.  Updegraff, G. E. and Anderson, V. C. Bubble noise and wavelet spills recorded 1m below the ocean surface. J. Acoust. Soc. Am. 1991. 89: p. 2264–2279. (doi:10.1121/1.400917) 11.  Leighton, T. G., White, P. R. and Schneider, M. F. The detection and dimension of bubble entrainment and comminution. J. Acoust. Soc. Am. 1998. 103: p.  1825–1835. (doi:10.1121/1.421374) 12.  Pumphrey, H. C. and Ffowcs Williams, J. E. Bubbles as sources of ambient noise. IEEE J. Ocean. Eng. 1990. 15: p.  268–274. (doi:10.1109/48.103520) 13. Nikolovska, A. and Waldmann, C. Passive acoustic quantification of underwater gas seepage. In OCEANS, Boston, 18–21 September 2006, p. 6. New York, NY: Institute of Electrical and Electronic Engineers. 2006 (doi:10.1109/OCEANS.2006.306926) 14. Greene, C.A. and P.S. Wilson, Laboratory investigation of a passive acoustic method for measurement of underwater gas seep ebullition. Journal of the Acoustical Society of America, 2012. 131(1): p. El61-El66. 15. Westbrook, G.K., K.E. Thatcher, E.J. Rohling, A.M. Piotrowski, H. Palike, A.H. Osborne, E.G. Nisbet, T.A. Minshull, M. Lanoiselle, R.H. James, V. Huhnerbach, D. Green, R.E. Fisher, A.J. Crocker, A. Chabert, C. Bolton, A. Beszczynska-Moller, C. Berndt, and A. Aquilina, Escape of methane gas from the seabed along the West Spitsbergen continental margin. Geophysical Research Letters, 2009. 36. 16. Vagle, S. and D.M. Farmer, The Measurement of Bubble-Size Distributions by Acoustical Backscatter. Journal of Atmospheric and Oceanic Technology, 1992. 9(5): p. 630-644. 17. Simmonds, E.J. and D.N. MacLennan, Fisheries acoustics : theory and practice. 2nd ed. Fish and aquatic resources series ;2005, Oxford ; Ames, Iowa: Blackwell Science. xvii, 437 p., [15] p. of plates. 18. Ainslie, M.A. and T.G. Leighton, Review of scattering and extinction cross-sections, damping factors, and resonance frequencies of a spherical gas bubble. Journal of the Acoustical Society of America, 2011. 130(5): p. 3184-3208. 19. Lebourges-Dhaussy, A., Caractérisation des populations planctoniques par acoustique multifréquence. Océmis, 1996. 22(1): p. 71-92.   152

Acoustic detection of seabed gas leaks, with application to carbon capture and storage (CCS), and leak prevention for the oil and gas industry: preliminary assessment of use of active and passive acoustic inversion for the quantification of underwater gas releases

Southampton (e-Prints Soton)

Proceedings of the 11th European Conference on Underwater Acoustics ACOUSTIC DETECTION OF SEABED GAS LEAKS, WITH APPLICATION  TO  CARBON  CAPTURE  AND  STORAGE (CCS), AND LEAK PREVENTION FOR THE OIL AND GAS INDUSTRY:  PRELIMINARY  ASSESSMENT  OF  USE  OF ACTIVE AND PASSIVE ACOUSTIC INVERSION FOR THE QUANTIFICATION OF UNDERWATER GAS RELEASES  B. J. P. Bergès Institute of Sound and Vibration Research, University of Southampton, UK  T. G. Leighton  Institute of Sound and Vibration Research, University of Southampton, UK P. R. White  Institute of Sound and Vibration Research, University of Southampton, UK M. Tomczyk  University of Bremen, Marum, Bremen, Germany I.C. Wright  National Oceanography Center, Southampton, United Kingdom  1  INTRODUCTION The  acoustic  remote  sensing  of  subsea  gas  leakage  is  becoming  increasingly  important.  This includes the monitoring of underwater discharges from human related and natural sources, for the following reasons. First, as the oil and gas industry faces increasing regulation from authorities, there is a need to put more control in the industrial process and to assess the impact of activities on the marine environment [1]. The applications are diverse, including: early warnings of “blow-out” from offshore installations, detection of leaks from underwater gas pipelines, gas leakage detection from Carbon and Capture and Storage facilities (a process aimed at mitigating the release of large quantities of     in the atmosphere), and seabed monitoring (for the stability of civil engineering project and prediction of underwater landslip) [1,2]. Second, this technology has a role to play in oceanography for a better understanding of natural occurrences of gas release from the seafloor such as gas seepage or mud volcanoes. This is of major importance for the assessment of the exchange of gas between the ocean and the atmosphere with application to global warming. All those phenomena involved the formation and release of bubbles of different sizes (from tiny bubble streams  to  large  bubble  clouds).  These  can  be  detected  acoustically  (using  passive  and  active acoustic techniques) because they are strong sources and scatterers of sound [3,4].  This  paper  reports  progress  to  date  on  an  ongoing  two-phase  study.  This  project  is  aimed  at assessing  the  accuracy  of  active  and  passive  acoustic  techniques  for  the  quantification  of  gas releases with application to methane seepage and gas leaks from pipelines.  First, water tank experiments consisting  of the release of clouds of bubbles were undertaken in order  to  estimate  acoustically  the  bubble  generation  rates  and  correlate  the  results  with independent measurement of flow rates. The acoustic emissions are monitored using calibrated hydrophones and post processed signals are used to infer the bubble populations using the model derived by Leighton and White [5]. The results are compared to assess the  application and the accuracy of the technique.  Second,  a  multifrequency  inversion  model  of  single  beam  echosounder  data  from  bubbles  is proposed. This model is applied to EK60 data collected during the JCR253 scientific cruise [6] that observed  bubble  plumes  formed  from  methane  seepage  venting  from  the  seabed  of  the  West Spitsbergen continental margin.  2  PASSIVE ACOUSTIC INVERSION 146Proceedings of the 11th European Conference on Underwater Acoustics   2.1  Procedure Measurements of passive acoustic emissions of bubble clouds were conducted in an 8 m x 8 m x 5 m deep test tank containing fresh water at 10°C. The bubble generation system used consisted on an arrangement of needles in circle on a plate. The spacing between them was approximately 3 cm and the size of each nozzle was 1.2 mm. A nitrogen gas cylinder was used to produce the gas for generating the bubbles. The output of the bottle was connected to a mass flow meter (Bronkhorst in-flow series, model F-111BI) adjusting the gas flow. The measurements of gas flow were recorded via a data acquisition system (DAQ). The bubble generation system was then connected to the end of the gas line and deployed at the bottom of the test tank.  For the acquisition of the acoustic signals, a calibrated T8105 B&K hydrophone was placed at a range of 5 meters from the base of the bubble cloud. This was connected to a B&K T2635 charge amplifier and a data acquisition unit.   Figure 1: schematic of the experimental apparatus. Bubbles were released using a nitrogen gas bottle and a bubbling system composed of six needles. The acoustic emissions were recording using a calibrated hydrophone and the flow rate was acquired using a mass flow meter connected to independent acquisition units.  The recorded signals were bandpass filtered and corrected to account for the reverberation of the enclosure. This correction is based on the theory by Cochard et al. [7] that expresses the emission in  free  field  from  given  measurements  in  a  reverberant  environment.  For  this  experiment,  the volume of the test tank is            and the reverberation time is             .  From the data collected by the hydrophone, the bubble size distributions are determined using the model by Leighton and White [5]. The power spectral density  ( ) of the signal can be expressed as:      ( )   ∫  (  )|  (    )|          (1)   147Proceedings of the 11th European Conference on Underwater Acoustics    with  |  (    )|  denoting  the  squared magnitude  of  the  Fourier  transform  of  the  response  of  a single bubble of radius   . The quantity  (  ) is the bubble-emission size distribution as a function of   , defined such that ∫  (  )         represents the number of bubbles generated per second with a radius in the range (     ).   This problem can be solved numerically as the equation defines a Fredholm integral of the first kind that can be discretized [5]. The determination of the bubble distributions consists on solving the inverse problem expressed in matrix form as:                (2)    The number of radius bins is chosen to be equal to the number of frequency bins in order to build a square  problem.  However,  the  problem  remains  ill-posed  which  means  that  the  inevitable measurement errors in  ( ) are magnified. Tikhonov regularisation is applied in order to achieve a positive and stable solution for  (  ). Assuming spherical bubbles, the flow rate is calculated as follows:             ∫  (  )            (3)    This gives the final results that are compared to the independent measures from the mass flow meter (suitable corrections being made for the hydrostatic pressure imparted by the ~5 m of water). The comparison is made for nine flow rate regimes covering more than an order of magnitude in gas flow rate.  2.2  Results  Figure 2: Comparison of different flow rates calculated at different regimes and plotted in a log scale. The values represented by the red curve with stars are the measurements from the mass flow meter. The black dotted line with squares is the flow rates inferred from the acoustic signal 148Proceedings of the 11th European Conference on Underwater Acoustics   generated by the needles system. The error bars represent the uncertainty resulting from the background noise of the recordings which represents                  when inverted.  The  gas  flow  rates  calculated  using  the  inversion  process  described  in  the  previous  section  is compared to measurements from the mass flow meter. The results for the nine regimes are shown in figure 2. Error bars show the uncertainty on the bubble count arising from the background noise. From this plot, it is noticeable that there is a good agreement at the highest flow rates. However, as the gas flux becomes smaller, the background noise contribution becomes increasingly significant compared to the bubble signal and so the difference with the mass flow meter measures becomes greater. The level calculated from the acoustic signals stabilizes when the flow rate becomes low (regimes 6-9) where the measurements are dominated by noise.  The model studied in this paper aim to quantify gas fluxes for large gas release events. However, for small events as observed by Leifer and Tang [8], presenting low flow rate, the model might not be  appropriate  because  when  individual  bubble  signatures  can  be  identified,  the  time  between these  signatures  contains  just  noise  and  as  these  intervals  become  longer,  noise  increasingly contributes to the spectrum. Identification of bubble generate rates in the natural world dates from the 1980s, and has been applied to waterfalls [9], ocean wave breaking [10], and rainfall over the ocean [11,12] and, more recently, explored to examine to bubble emissions from seeps [8, 13,14]. A combination of the two techniques possibly offers a good cover of flow rate ranges.    3  ACTIVE ACOUSTIC INVERSION During JR253 cruise on August 2011 to the West Spitsbergen region, areas that exhibited strong methane venting during JR211 cruise [15] were investigated. In addition new gas plumes have been discovered in shallow depth regions (range of 80-100 m). The acoustic surveys were conducted using an EK60 single beam multifrequency echosounder scanning at three frequencies: 38 kHz, 120 kHz and 200 kHz. As the EK60 is a calibrated system, scattering cross-section per unit volume    could be calculated from the raw data and an example is show in figure 3. The echograms at three  frequencies  are  presented  and  strong  bubble  plumes  escaping  from  the  seafloor  can  be observed at 5 minutes time. In this study, those echo levels are used to infer bubble abundances using an inversion technique based on the study by Vagle and Farmer [16], similar to methods used in fisheries acoustics for the calculation of fish densities [17].   Depending  on  the  frequency,  a  gas  bubble  is  responding  differently  to  an  acoustic  field.  More specifically, the scattering behaviour of an object can be described by it scattering cross section   . In the specific case of a spherical gas bubble, the theory was recently reviewed by Ainslie and Leighton [18] and  is used for the calculation of    in this study. The difference of echo level at different frequencies is directly related to the density of bubbles of different sizes and is used to calculate bubble abundances. At a frequency    , the backscattering volume expressed as inverse meter (   ) is related to the bubble distribution as followed:          ∫   (      )  (  )        (4)    with  (  )  the  bubble  size  distribution  expressed  in  number  of  bubbles  per  cubic  meters.  This equation defines a Fredholm integral of the first kind that can be discretized. The determination of  (  ) consists on solving the following inverse problem expressed in matrix form:                 (5)    149Proceedings of the 11th European Conference on Underwater Acoustics   Using the data collected by the EK60, inversion is performed using backscattering volume levels from the bubble plumes at different frequencies from data set as presented in figure 3. The number of radius bins is chosen to be equal to the number of frequency bins in order to build a square problem. This problem also tends to be ill-posed because of inevitable errors in    and Tikhonov regularization is applied to control the growth of errors. The result of using such an approach will be a bubble size distribution based on the bubble in three frequency bins only, as the EK60 system gives  echo  levels  at  38  kHz,  120  kHz  and  200  kHz.  Algorithms  such  as  the  one  described  by Lebourges-Dhaussy  [19]  that  is  used  for  zooplankton  classification  seem  to  be  well  suited  for solving the problem stated in this study with increased number of radius bins while having a low number of frequency bins. a)   b)   150Proceedings of the 11th European Conference on Underwater Acoustics   c)    Figure 3: this figure shows echograms from data collected during JCR253 scientific cruise using the EK60 single beam multifrequency echosounder. From the top to the bottom, the frequencies are a) 38 kHz, b) 120 kHz, c) 200 kHz. The scattering cross-sections per unit volume    are plotted versus time (minutes) and depth (meter). Strong bubble plumes can be observed, starting at 5 minutes time.    4  CONCLUSION Active and passive acoustic measurements were performed and presented in this paper. First, the accuracy of a passive acoustic inversion model for the quantification of high flow rate gas leaks proposed by Leighton and White [5] was studied. Comparisons were made between measures from a  calibrated  hydrophone  and  a  mass  flow  meter.  Second,  a  three  point  inversion  technique  is presented with data it can be applied to.  ACKNOWLEDGEMENTS The  studentship  of  Mr  Bergès  is  sponsored  by  Statoil  Ltd.  The  studentship  of  Mr.  Tomczyk  is sponsored by the SENSEnet project within an EU Framework 7 funded Marie Curie Initial Training Network. The data from the JCR253 scientific cruise presented in this report belong to the National Oceanography Centre, Southampton, UK. The authors thank Dr Trond Erland Bustnes of Statoil for providing guidance on industrial practicalities and requirements.  REFERENCES   1.  Chris, T., Subsea leak detection. Exploration & Production, 2007. 6(1). 2.  Leighton, T.G.,  Theory for acoustic propagation in marine sediment containing gas bubbles which may pulsate in a non-stationary nonlinear manner, Geophysical Research Letters, 2007. 34: L17607 3.  Leighton, T.G., The acoustic bubble1994, London: Academic Press. xxvi, 613 p. 4.  Ainslie, M.A. and Leighton, T.G. Near resonant bubble acoustic cross-section corrections, including examples from oceanography, volcanology, and biomedical ultrasound, Journal of the Acoustical Society of America, 2009. 126(5): p. 2163-2175. 5.  Leighton, T.G. and P.R. White, Quantification of undersea gas leaks from carbon capture and storage facilities, from pipelines and from methane seeps, by their acoustic emissions. 151Proceedings of the 11th European Conference on Underwater Acoustics   Proceedings of the Royal Society a-Mathematical Physical and Engineering Sciences, 2012. 468(2138): p. 485-510. 6.   JR253 cruise plan. Lastly visited: 30/04/2012 http://www.antarctica.ac.uk/documents/cruise/JCR253%20Cruise%20Plan_compressed.pdf 7.   Cochard, N., J.L. Lacoume, P. Arzelies, and Y. Gabillet, Underwater acoustic noise measurement in test tanks. Ieee Journal of Oceanic Engineering, 2000. 25(4): p. 516-522. 8.  Leifer, I. and D.J. Tang, The acoustic signature of marine seep bubbles. Journal of the Acoustical Society of America, 2007. 121(1): p. El35-El40. 9.   Leighton, T. G. and Walton, A. J. An experimental study of the sound emitted from gas bubbles in a liquid. Eur. J. Phys.  1987. 8: p. 98–104. (doi:10.1088/0143-0807/8/2/005) 10.   Updegraff, G. E. and Anderson, V. C. Bubble noise and wavelet spills recorded 1m below the ocean surface. J. Acoust. Soc. Am. 1991. 89: p. 2264–2279. (doi:10.1121/1.400917) 11.   Leighton, T. G., White, P. R. and Schneider, M. F. The detection and dimension of bubble entrainment and comminution. J. Acoust. Soc. Am. 1998. 103: p.  1825–1835. (doi:10.1121/1.421374) 12.   Pumphrey, H. C. and Ffowcs Williams, J. E. Bubbles as sources of ambient noise. IEEE J. Ocean. Eng. 1990. 15: p.  268–274. (doi:10.1109/48.103520) 13.  Nikolovska, A. and Waldmann, C. Passive acoustic quantification of underwater gas seepage. In OCEANS, Boston, 18–21 September 2006, p. 6. New York, NY: Institute of Electrical and Electronic Engineers. 2006 (doi:10.1109/OCEANS.2006.306926) 14.  Greene, C.A. and P.S. Wilson, Laboratory investigation of a passive acoustic method for measurement of underwater gas seep ebullition. Journal of the Acoustical Society of America, 2012. 131(1): p. El61-El66. 15.  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An experimental study of the sound emitted from gas bubbles in a liquid.

Bubble noise and wavelet spills recorded 1m below the ocean surface.

Bubbles as sources of ambient noise.

Caractérisation des populations planctoniques par acoustique multifréquence. Océmis,

Escape of methane gas from the seabed along the West Spitsbergen continental margin. Geophysical Research Letters,

Fisheries acoustics : theory and practice. 2nd ed. Fish and aquatic resources series ;2005,

Laboratory investigation of a passive acoustic method for measurement of underwater gas seep ebullition.

Near resonant bubble acoustic cross-section corrections, including examples from oceanography, volcanology, and biomedical ultrasound,

Passive acoustic quantification of underwater gas seepage.

Quantification of undersea gas leaks from carbon capture and storage facilities, from pipelines and from methane seeps, by their acoustic emissions.

Review of scattering and extinction cross-sections, damping factors, and resonance frequencies of a spherical gas bubble.

Subsea leak detection. Exploration & Production,

The acoustic bubble1994,

The acoustic signature of marine seep bubbles.

The detection and dimension of bubble entrainment and comminution.

The Measurement of Bubble-Size Distributions by Acoustical Backscatter.

Theory for acoustic propagation in marine sediment containing gas bubbles which may pulsate in a non-stationary nonlinear manner,

Underwater acoustic noise measurement in test tanks.

http://nora.nerc.ac.uk/441713/1/Pub12705.pdf

Acoustic detection of seabed gas leaks, with application to carbon capture and storage (CCS), and leak prevention for the oil and gas industry: preliminary assessment of use of active and passive acoustic inversion for the quantification of underwater gas releases

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