Bulk diamond phonons have been shown to be a versatile platform for the
generation, storage, and manipulation of high-bandwidth quantum states of
light. Here we demonstrate a diamond quantum memory that stores, and releases
on demand, an arbitrarily polarized ∼250 fs duration photonic qubit. The
single-mode nature of the memory is overcome by mapping the two degrees of
polarization of the qubit, via Raman transitions, onto two spatially distinct
optical phonon modes located in the same diamond crystal. The two modes are
coherently recombined upon retrieval and quantum process tomography confirms
that the memory faithfully reproduces the input state with average fidelity
0.784±0.004 with a total memory efficiency of (0.76±0.03)%. In an
additional demonstration, one photon of a polarization-entangled pair is stored
in the memory. We report that entanglement persists in the retrieved state for
up to 1.3 ps of storage time. These results demonstrate that the diamond phonon
platform can be used in concert with polarization qubits, a key requirement for
polarization-encoded photonic processing