The structural integrity of vacuumatics relies on the principle of prestressing unbound particles inside an enclosed membrane. By introducing a negative pressure (partial vacuum) inside this airtight flexible enclosure, the membrane is tightly wrapped around the outer particles, hence effectively bonding the particle filling to create (adaptable) load-bearing structures. Analytical and numerical studies on the fundamental prestress derivation of vacuumatically prestressed structures have shown that the effective prestressing forces between the particles largely depend, apart from the differential in (air) pressure differential, on the elastic properties of the skin material. The flexural rigidity of vacuumatics is mainly determined by the material properties of the particles and membrane used. Variations in elasticity of the skin and particle filling, and with this the shape, size, compressiveness, roughness, and packing density of the individual particles, highly influence the structural behaviour of vacuumatic structures. In order to explore the influence of different particle and skin characteristics (or parameters) on the flexural rigidity, experimental research has been carried out by means of four point bending tests. Different types of particles were used to discover behavioural trends dependent on the parameters varied. The results of this study provide an enhanced understanding of the true overall structural response of vacuumatics. By systematically elaborating the different parameters, we are able to determine what specific material properties are desired to design the ‘most efficient’ vacuumatic structure for every application