Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Physics, 2011.Cataloged from PDF version of thesis.Includes bibliographical references (p. 218-226).The thesis presents results from experiments in which ultracold Sodium-6 and Lithium-23 atomic gases were studied near a Feshbach resonance at high magnetic fields. The enhanced interactions between atoms in the presence of a molecular state enhance collisions, leading to inelastic decay and loss, many-body dynamics, novel quantum phases, and molecule formation. Experimental data is presented alongside relevant theory and numerical models. Results are presented for both homonuclear Na 2 and Li 2 molecules, as well as heteronuclear NaLi resonances, although we were unable to isolate and measure NaLi molecules. Furthermore, experiments and theories related to strongly-correlated quantum phases such as Stoner model ferromagnetism, Bose mediated Fermi interactions, and Bose-Fermi mixtures are presented as applicable to Na and Li gases. Conclusions are presented regarding the feasibility of producing deeply bound, dipolar NaLi molecules, as well as future prospects for strongly interacting atomic gases of Na and Li.by Caleb A. Christensen.Ph.D
