Above-Room-Temperature Ferromagnetic Ni2+:ZnO Thin Films Prepared from Colloidal Diluted Magnetic Semiconductor Quantum Dots

Abstract

We report the preparation of spin-coated nickel-doped zinc oxide nanocrystalline thin films using high-quality colloidal diluted magnetic semiconductor (DMS) quantum dots as solution precursors. These films show robust ferromagnetism with Curie temperatures above 350 K and 300 K saturation moments up to 0.1 Bohr magnetons per nickel. These results demonstrate a step toward the use of colloidal zero-dimensional DMS nanocrystals as building blocks for the bottom-up construction of more complex ferromagnetic semiconductor nanostructures

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