We report efficient terahertz (THz) generation in epitaxial
α-W/Co6​0Fe4​0 spintronic emitters. Two types of emitters have been
investigated; epitaxial α-W(110)/Co6​0Fe4​0(110) and
α-W(001)/Co6​0Fe4​0(001) deposited on single crystalline
Al2​O3​(11-20) and MgO(001) substrates, respectively. The generated THz
radiation is about 10% larger for α-W(110)/Co6​0Fe4​0(110) grown on
single crystalline Al2​O3​(11-20), which is explained by the fact that the
α-W(110)/Co6​0Fe4​0(110) interface for this emitter is more
transparent to the spin current due to the presence of Angstrom-scale interface
intermixing at the W/CoFe interface. Our results also reveal that the
generation of THz radiation is larger when pumping with the laser light from
the substrate side, which is explained by a larger part of the laser light due
to interference effects in the film stack being absorbed in the ferromagnetic
Co6​0Fe4​0 layer in this measurement configuration