Static magnetic order with strong quantum fluctuations in spin-1/2 honeycomb magnet Na2Co2TeO6

Abstract

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev interactions typically promote a zigzag antiferromagnetic order in the d-orbital transition metal compounds. By combining neutron scattering with muon-spin rotation and relaxation techniques, we provide new insights into the exotic properties of Na2Co2TeO6, a candidate Kitaev material. Below TN, the zero-field muon-spin relaxation rate becomes almost constant (at 0.45 us-1). We attribute this temperature-independent muon-spin relaxation rate to the strong quantum fluctuations, as well as to the frustrated Kitaev interactions. As the magnetic field increases, neutron scattering data indicate a much broader spin-wave-excitation gap at the K-point. Therefore, quantum fluctuations seem not only robust, but are even enhanced by the applied magnetic field. Our findings provide valuable hints for understanding the onset of the quantum-spin-liquid state in Kitaev materials.Comment: 28 pages, 11 figures, and 1 labl