Demonstration and frequency noise characterization of a 17 $\mu$m quantum cascade laser

Abstract

We describe the properties of a continuous-wave room-temperature quantum cascade laser operating at the long wavelength of 17 $\mu$m. Long wavelength mid-infrared quantum cascade lasers offer new opportunities for chemical detection, vibrational spectroscopy and metrological measurements using molecular species. In particular, probing low energy vibrational transitions would be beneficial to the spectroscopy of large and complex molecules, reducing intramolecular vibrational energy redistribution which acts as a decoherence channel. By performing linear absorption spectroscopy of the v2 fundamental vibrational mode of N2O molecules, we have demonstrated the spectral range and spectroscopic potential of this laser, and characterized its free-running frequency noise properties. Finally, we also discuss the potential application of this specific laser in an experiment to test fundamental physics with ultra-cold molecules