A high-spin nucleus coupled to a color center can act as a long-lived memory
qudit in a spin-photon interface. The germanium vacancy (GeV) in diamond has
attracted recent attention due to its excellent spectral properties and
provides access to the 10-dimensional Hilbert space of the I=9/273Ge nucleus. Here, we observe the 73GeV hyperfine structure,
perform nuclear spin readout, and optically initialize the 73Ge spin
into any eigenstate on a μs-timescale and with a fidelity of up to 97±3%. Our results establish 73GeV as an optically addressable high-spin
quantum platform for a high-efficiency spin-photon interface as well as for
foundational quantum physics and metrology.Comment: 8 pages, 4 figure