Lifshitz transition enabling superconducting dome around the quantum critical point in TiSe2_2

Abstract

Superconductivity often emerges as a dome around a quantum critical point (QCP) where long-range order is suppressed to zero temperature. So far, this has been mostly studied in magnetically ordered materials. By contrast, the interplay between charge order and superconductivity at a QCP is not fully understood. Here, we present resistance measurements proving that a dome of superconductivity surrounds the charge-density-wave (CDW) QCP in pristine samples of 1TT-TiSe2_2 tuned with hydrostatic pressure. Furthermore, we use quantum oscillation measurements to show that the superconductivity sets in at a Lifshitz transition in the electronic band structure. We use density functional theory to identify the Fermi pockets enabling superconductivity: large electron and hole pockets connected by the CDW wave vector Q⃗\vec{Q} which emerge upon partial suppression of the zero-pressure CDW gap. Hence, we conclude that superconductivity is of interband type enabled by the presence of hole and electron bands connected by the CDW Q⃗\vec{Q} vector. Earlier calculations show that interband interactions are repulsive, which suggests that unconventional s±_{\pm} superconductivity is realised in TiSe2_2 - similar to the iron pnictides. These results highlight the importance of Lifshitz transitions in realising unconventional superconductivity and help understand its interaction with CDW order in numerous materials.Comment: 21 pages, 5 figure

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