Although compliance allows the soft robot to be under-actuated and generalise its control, it also impacts the ability of the robot to exert forces on the environment. There is a trade-off between robots being compliant or precise and strong. Many mechanisms that change robots' stiffness on demand have been proposed, but none are perfect, usually compromising the device's compliance and restricting its motion capabilities. Keeping the above issues in mind, this thesis focuses on creating robust and reliable pneumatic actuators, that are designed to be easily manufactured with simple tools. They are optimised towards linear behaviour, which simplifies modelling and improve control strategies. The principle idea in relation to linearisation is a reinforcement strategy designed to amplify the desired, and limit the unwanted, deformation of the device. Such reinforcement can be achieved using fibres or 3D printed structures. I have shown that the linearity of the actuation is, among others, a function of the reinforcement density and shape, in that the response of dense fibre-reinforced actuators with a circular cross-section is significantly more linear than that of non-reinforced or non-circular actuators. I have explored moulding manufacturing techniques and a mixture of 3D printing and moulding. Many aspects of these techniques have been optimised for reliability, repeatability, and process simplification. I have proposed and implemented a novel moulding technique that uses disposable moulds and can easily be used by an inexperienced operator. I also tried to address the compliance-stiffness trade-off issue. As a result, I have proposed an intelligent structure that behaves differently depending on the conditions. Thanks to its properties, such a structure could be used in applications that require flexibility, but also the ability to resist external disturbances when necessary. Due to its nature, individual cells of the proposed system could be used to implement physical logic elements, resulting in embodied intelligent behaviours. As a proof-of-concept, I have demonstrated use of my actuators in several applications including prosthetic hands, octopus, and fish robots. Each of those devices benefits from a slightly different actuation system but each is based on the same core idea - fibre reinforced actuators. I have shown that the proposed design and manufacturing techniques have several advantages over the methods used so far. The manufacturing methods I developed are more reliable, repeatable, and require less manual work than the various other methods described in the literature. I have also shown that the proposed actuators can be successfully used in real-life applications. Finally, one of the most important outcomes of my research is a contribution to an orthotic device based on soft pneumatic actuators. The device has been successfully deployed, and, at the time of submission of this thesis, has been used for several months, with good results reported, by a patient