Layered Mott insulator α-RuCl3​ has been intensely investigated
as a possible candidate for Kitaev quantum spin liquid. In this letter, we
report electron tunneling measurements on few-layer α-RuCl3​ in
proximity to graphite, using a scanning tunneling microscopy. Signatures of
charge doping have been observed in α-RuCl3​ layers stacking on
the surface of graphite. Upon charge doping, we observed characteristic
tunneling spectra that are dependent on the number of layers of
α-RuCl3​. For a single α-RuCl3​ layer that is in
direct contact with graphite, data shows charge states emerging in the Mott-gap
regime with conservation of the Hubbard bands. For a bilayer of
α-RuCl3​, data indicates an unconventional Mott-phase transition,
where the Hubbard bands collapse accompanied by a dramatical gap-reduction. The
results have thus demonstrated that tunneling into doped few-layer
α-RuCl3​ is a useful probe to investigate this otherwise
insulating spin-liquid candidate, providing fundamental information concerning
electronic properties and theoretically proposed strong correlation physics in
α-RuCl3​.Comment: Original data are available upon resonable request from corresponding
autho