Kinetic theory of the nonlocal electrodynamic response in anisotropic metals: Skin effect in 2D systems

Abstract

The electrodynamic response of ultrapure materials at low temperatures becomes spatially nonlocal. This nonlocality gives rise to phenomena such as hydrodynamic flow in transport and the anomalous skin effect in optics. In systems characterized by an anisotropic electronic dispersion, the nonlocal dynamics becomes dependent on the relative orientation of the sample with respect to the applied field, in ways that go beyond the usual, homogeneous response. Such orientational dependence should manifest itself not only in transport experiments, as recently observed, but also in optical spectroscopy. In this paper, we develop a kinetic theory for the distribution function and the transverse conductivity of two- and three-dimensional Fermi systems with anisotropic electronic dispersion. By expanding the collision integral into the eigenbasis of a collision operator, we include momentum-relaxing scattering as well as momentum-conserving collisions. We examine the isotropic 2D case as a reference, as well as anisotropic hexagonal and square Fermi-surface shapes. We apply our theory to the quantitative calculation of the skin depth and the surface impedance, in all regimes of skin effect. We find qualitative differences between the frequency dependence of the impedance in isotropic and anisotropic systems. Such differences are shown to persist even for more complex 2D Fermi surfaces, including the “supercircle” geometry and an experimental parametrization for PdCoO2_2, which deviate from an ideal polygonal shape. We study the orientational dependence of skin effect due to Fermi-surface anisotropy, thus providing guidance for the experimental study of nonlocal optical effects

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