Revealing a spatially inhomogeneous broadening effect in artificial quantum structures caused by electron-adsorbate scattering

Abstract

What defines the lifetime of electronic states in artificial quantum structures? We measured the spectral widths of resonant eigenstates in a circular, CO-based quantum corral on a Cu(111) surface and found that the widths are related to the size of the corral and that the line shape is essentially Gaussian. A model linking the energy dependence with the movement of single surface electrons shows that the observed behavior is consistent with lifetime limitations due to interaction with the corral walls