We demonstrate a nonlinear Hall effect due to the boundary spin accumulation
in Pt films grown on Al2O3 substrates. This Hall effect and the previously
demonstrated Hanle magnetoresistance provide a complete picture of the
spin-precession control of the spin and charge transport at the boundary of a
spin-orbit coupled material, which we refer to as spin-Hall Hanle effects
(SHHE). We also show that the SHHE can be employed to measure the spin
diffusion length, the spin-Hall angle, and the spin relaxation time of heavy
metal without the need of magnetic interface or the input from other
measurements. The comprehensive demonstration of SHHE in such a simple system
suggests they may be ubiquitous and needs to be considered for unravelling the
spin and charge transport in more complex thin film structures of spin-orbit
coupled materials