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Towards time resolved core level photoelectron spectroscopy with femtosecond x-ray free-electron lasers
Authors
M. Beye
M. Deppe
+9 more
K. Dörich
A. Föhlisch
C. Gahl
F. Hennies
A. Melnikov
M. Nagasono
A. Pietzsch
E. Suljotil
W. Wurth
Publication date
1 January 2008
Publisher
College Park, MD : Institute of Physics Publishing
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Abstract
We have performed core level photoelectron spectroscopy on a W(110) single crystal with femtosecond XUV pulses from the free-electron laser at Hamburg (FLASH). We demonstrate experimentally and through theoretical modelling that for a suitable range of photon fluences per pulse, time-resolved photoemission experiments on solid surfaces are possible. Using FLASH pulses in combination with a synchronized optical laser, we have performed femtosecond time-resolved core-level photoelectron spectroscopy and observed sideband formation on the W 4f lines indicating a cross correlation between femtosecond optical and XUV pulses. © IOP Publishing Ltd and Deutsche Physikalische Gesellschaft
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Last time updated on 23/07/2022