This paper presents the integration of electrical capacitance tomography (ECT) with a moisture controller for the microwave drying of polymer foam. The proportional–integral (PI) control and the linear quadratic Gaussian (LQG) control are employed in designing the controller. The control objective in this process is that the moisture of polymer foam after the drying process reaches the desired set point. The permittivity distribution of polymer foam after the drying process is estimated in real-time using a designed ECT sensor and transferred as feedback to the controller. Since the permittivity and the moisture are strongly correlated, the material moisture can be controlled by controlling the permittivity. A state-space model is derived for the microwave drying process based on a system identification approach using the experimental data from the process. The derived model is employed in designing the LQG controller and adjusting the parameters of the PI controller. The designed controllers are implemented on a testbed microwave oven, and the experimental results show that the designed controllers are able to follow the desired set point moisture. The performance of the system with both controllers is compared, and their advantages and disadvantages are discussed. Moreover, the benefits of having a moisture controller for the microwave drying process are shown in simulation studies compared to an uncontrolled system