Complete and precise characterization of a quantum dynamical process can be
achieved via the method of quantum process tomography. Using a source of
correlated photons, we have implemented several methods investigating a wide
range of processes, e.g., unitary, decohering, and polarizing. One of these
methods, ancilla-assisted process tomography (AAPT), makes use of an additional
``ancilla system,'' and we have theoretically determined the conditions when
AAPT is possible. All prior schemes for AAPT make use of entangled states. Our
results show that, surprisingly, entanglement is not required for AAPT, and we
present process tomography data obtained using an input state that has no
entanglement. However, the use of entanglement yields superior results.Comment: To appear in Physical Review Letter
