The frequency comb created by a femtosecond mode-locked laser and a
microstructured fiber is used to phase coherently measure the frequencies of
both the Hg^+ and Ca optical standards with respect to the SI second as
realized at NIST. We find the transition frequencies to be f_Hg=1 064 721 609
899 143(10) Hz and f_Ca=455 986 240 494 158(26) Hz, respectively. In addition
to the unprecedented precision demonstrated here, this work is the precursor to
all-optical atomic clocks based on the Hg^+ and Ca standards. Furthermore, when
combined with previous measurements, we find no time variations of these atomic
frequencies within the uncertainties of |(df_Ca/dt)/f_Ca| < 8 x 10^{-14}
yr^{-1}, and |(df_Hg/dt)/f_Hg|< 30 x 10^{-14} yr^{-1}.Comment: 6 pages, including 4 figures. RevTex 4. Submitted to Phys. Rev. Let
