Light controlled photon tunneling

Recent measurements of photon tunneling through individual subwavelength pinholes in a gold film covered with a layer of polydiacetylene (Phys. Rev. Letters 88, 187402 (2002)) provided strong indication of "photon blockade" effect similar to Coulomb blockade phenomenon observed in single-electron tunneling experiments. Here we report first observation of photon tunneling been blocked (gated) by light at a different wavelength. This observation suggests possibility of building new class of photon tunneling gating devices for all-optical signal processing.Comment: 11 pages, 3 figure

Nonlocal Optics of Plasmonic Nanowire Metamaterials

We present an analytical description of the nonlocal optical response of plasmonic nanowire metamaterials that enable negative refraction, subwavelength light manipulation, and emission lifetime engineering. We show that dispersion of optical waves propagating in nanowire media results from coupling of transverse and longitudinal electromagnetic modes supported by the composite and derive the nonlocal effective medium approximation for this dispersion. We derive the profiles of electric field across the unit cell, and use these expressions to solve the long-standing problem of additional boundary conditions in calculations of transmission and reflection of waves by nonlocal nanowire media. We verify our analytical results with numerical solutions of Maxwell's equations and discuss generalization of the developed formalism to other uniaxial metamaterials

Shaping plasmon beams via the controlled illumination of finite-size plasmonic crystals

Plasmonic crystals provide many passive and active optical functionalities, including enhanced sensing, optical nonlinearities, light extraction from LEDs and coupling to and from subwavelength waveguides. Here we study, both experimentally and numerically, the coherent control of SPP beam excitation in finite size plasmonic crystals under focussed illumination. The correct combination of the illuminating spot size, its position relative to the plasmonic crystal, wavelength and polarisation enables the efficient shaping and directionality of SPP beam launching. We show that under strongly focussed illumination, the illuminated part of the crystal acts as an antenna, launching surface plasmon waves which are subsequently filtered by the surrounding periodic lattice. Changing the illumination conditions provides rich opportunities to engineer the SPP emission pattern. This offers an alternative technique to actively modulate and control plasmonic signals, either via micro- and nano-electromechanical switches or with electro- and all-optical beam steering which have direct implications for the development of new integrated nanophotonic devices, such as plasmonic couplers and switches and on-chip signal demultiplexing. This approach can be generalised to all kinds of surface waves, either for the coupling and discrimination of light in planar dielectric waveguides or the generation and control of non-diffractive SPP beams

Influence of Photoexcitation Depth on Luminescence Spectra of Bulk GaAs Single Crystals and Defect Structure Characterization

The results of investigation of bulk GaAs photoluminescence are presented taken from near-surface layers of different thicknesses using for excitation the light with the wavelengths which are close but some greater than the excitonic absorption resonances (so-called bulk photoexcitation). Only the excitonic and band-edge luminescence is seen under the interband excitation, while under the bulk excitation, the spectra are much more informative. The interband excited spectra of all the samples investigated in the present work are practically identical, whereas the bulk excited PL spectra are different for different samples and excitation depths and provide the information on the deep-level point defect composition of the bulk materials.Comment: Aalborg Summer School on Nonlinear Optics, Aalborg, Denmark, 7-12 August 199

Near-field polarization conversion in planar chiral nanostructures

Enantiomeric-sensitive optical polarization conversion has been observed in the near-field above a planar chiral nanostructures consisting of an array of gammadions cut in a metal film. Formation of the far-field scattered light rotated with respect to the incident linear polarized light has been visualized

Validation of the spectrophotometric method of determination of drug substance in medicine “Chloropyraminum, cream”

The article is devoted to validation of method of quantitative determination of drug substance – chloropyramine in medicine “Chloropiraminum, cream for external application, 10 mg/g”. The research purpose was to conf irm documentarily that a spectrophotometric method is suitable for quantitative determination of chloropyramine hydrochloride in medicine “Chloropyraminum, cream for external application, 10 mg/g” and allows getting results with the required metrology characteristics. The research objects were the samples of medicine “Chloropyraminum, cream fo r external application, 10 mg/g”. The absorbance measurements were conducted at the spectrophotometer of RV 2201A. It was developed the plan of validation, including the determination of the following validation characteristics: selectivity, trueness, application range, linearity and precision (repeatability and repro-ducibility within the laboratory). For every validation characteristic the criteria of acceptability were calculated. In accordance with the developed plan the experimental researches were carried out and it was found out that validation characteristics were in the accordance with th e criteria of acceptability. As a result of validation which was carried out in accordance with TKP 030-2013 (02040) it was con-firmed that spectrophotometric method for determination of chloropyramine hydrochloride in medicine “Chloropyraminum, cream for external application, 10 mg/g” is available

Magnetic dipole radiation tailored by substrates: numerical investigation

Nanoparticles of high refractive index materials can possess strong magnetic polarizabilities and give rise to artificial magnetism in the optical spectral range. While the response of individual dielectric or metal spherical particles can be described analytically via multipole decomposition in the Mie series, the influence of substrates, in many cases present in experimental observations, requires different approaches. Here, the comprehensive numerical studies of the influence of a substrate on the spectral response of high- index dielectric nanoparticles were performed. In particular, glass, perfect electric conductor, gold, and hyperbolic metamaterial substrates were investigated. Optical properties of nanoparticles were characterized via scattering cross-section spectra, electric field profiles, and induced electric and magnetic moments. The presence of substrates was shown to introduce significant impact on particle's magnetic resonances and resonant scattering cross-sections. Variation of substrate material provides an additional degree of freedom in tailoring properties of emission of magnetic multipoles, important in many applications.Comment: 10 page, 28 figure

Scattering Suppression from Arbitrary Objects in Spatially-Dispersive Layered Metamaterials

Concealing objects by making them invisible to an external electromagnetic probe is coined by the term cloaking. Cloaking devices, having numerous potential applications, are still face challenges in realization, especially in the visible spectral range. In particular, inherent losses and extreme parameters of metamaterials required for the cloak implementation are the limiting factors. Here, we numerically demonstrate nearly perfect suppression of scattering from arbitrary shaped objects in spatially dispersive metamaterial acting as an alignment-free concealing cover. We consider a realization of a metamaterial as a metal-dielectric multilayer and demonstrate suppression of scattering from an arbitrary object in forward and backward directions with perfectly preserved wavefronts and less than 10% absolute intensity change, despite spatial dispersion effects present in the composite metamaterial. Beyond the usual scattering suppression applications, the proposed configuration may serve as a simple realisation of scattering-free detectors and sensors

Tailoring and enhancing spontaneous two-photon emission processes using resonant plasmonic nanostructures

The rate of spontaneous emission is known to depend on the environment of a light source, and the enhancement of one-photon emission in a resonant cavity is known as the Purcell effect. Here we develop a theory of spontaneous two-photon emission for a general electromagnetic environment including inhomogeneous dispersive and absorptive media. This theory is used to evaluate the two-photon Purcell enhancement in the vicinity of metallic nanoparticles and it is demonstrated that the surface plasmon resonances supported by these particles can enhance the emission rate by more than two orders of magnitude. The control over two-photon Purcell enhancement given by tailored nanostructured environments could provide an emitter with any desired spectral response and may serve as an ultimate route for designing light sources with novel properties