Negative-Index Metamaterials: Second-Harmonic Generation, Manley-Rowe Relations and Parametric Amplification

Second harmonic generation and optical parametric amplification in negative-index metamaterials (NIMs) are studied. The opposite directions of the wave vector and the Poynting vector in NIMs results in a "backward" phase-matching condition, causing significant changes in the Manley-Rowe relations and spatial distributions of the coupled field intensities. It is shown that absorption in NIMs can be compensated by backward optical parametric amplification. The possibility of distributed-feedback parametric oscillation with no cavity has been demonstrated. The feasibility of the generation of entangled pairs of left- and right-handed counter-propagating photons is discussed.Comment: 7 pages, 6 figure

Quantum interference in nanofractals and its optical manifestation

We consider quantum interferences of ballistic electrons propagating inside fractal structures with nanometric size of their arms. We use a scaling argument to calculate the density of states of free electrons confined in a simple model fractal. We show how the fractal dimension governs the density of states and optical properties of fractal structures in the RF-IR region. We discuss the effect of disorder on the density of states along with the possibility of experimental observation.Comment: 19 pages, 6 figure

Second Harmonic Generation for a Dilute Suspension of Coated Particles

We derive an expression for the effective second-harmonic coefficient of a dilute suspension of coated spherical particles. It is assumed that the coating material, but not the core or the host, has a nonlinear susceptibility for second-harmonic generation (SHG). The resulting compact expression shows the various factors affecting the effective SHG coefficient. The effective SHG per unit volume of nonlinear coating material is found to be greatly enhanced at certain frequencies, corresponding to the surface plasmon resonance of the coated particles. Similar expression is also derived for a dilute suspension of coated discs. For coating materials with third-harmonic (THG) coefficient, results for the effective THG coefficients are given for the cases of coated particles and coated discs.Comment: 11 pages, 3 figures; accepted for publication in Phys. Rev.

Controlling Silver Nanoparticle Size and Morphology with Photostimulated Synthesis

Photo-induced synthesis and control over the size and shape of colloidal silver nanoparticles is investigated in contrast to photo-stimulated aggregation of small nanoparticles into large fractal-type structures. The feasibility of light-driven nanoengineering which enables manipulation of the sizes and shapes of the isolated nanoparticles is studied by varying the amount and type of the stabilizing agent and the type of optical irradiation.Comment: 10 pages, 7 figures, 11 image

Dimensional Crossover in the Effective Second Harmonic Generation of Films of Random Dielectrics

The effective nonlinear response of films of random composites consisting of a binary composite with nonlinear particles randomly embedded in a linear host is theoretically and numerically studied. A theoretical expression for the effective second harmonic generation susceptibility, incorporating the thickness of the film, is obtained by combining a modified effective-medium approximation with the general expression for the effective second harmonic generation susceptibility in a composite. The validity of the thoretical results is tested against results obtained by numerical simulations on random resistor networks. Numerical results are found to be well described by our theory. The result implies that the effective-medium approximation provides a convenient way for the estimation of the nonlinear response in films of random dielectrics.Comment: 9 pages, 2 figures; accepted for publication in Phys. Rev.

Fabricating plasmonic components for nanophotonics:[invited]

We report on experimental realization of different metal-dielectric structures that are used as surface plasmon polariton waveguides and as plasmonic metamaterials. Fabrication approaches based on different lithographic and deposition techniques are discussed

A concentration phenomenon for semilinear elliptic equations

For a domain \Omega\subset\dR^N we consider the equation -\Delta u + V(x)u = Q_n(x)\abs{u}^{p-2}u with zero Dirichlet boundary conditions and $p\in(2,2^*)$. Here $V\ge 0$ and $Q_n$ are bounded functions that are positive in a region contained in $\Omega$ and negative outside, and such that the sets $\{Q_n>0\}$ shrink to a point $x_0\in\Omega$ as $n\to\infty$. We show that if $u_n$ is a nontrivial solution corresponding to $Q_n$, then the sequence $(u_n)$ concentrates at $x_0$ with respect to the $H^1$ and certain $L^q$-norms. We also show that if the sets $\{Q_n>0\}$ shrink to two points and $u_n$ are ground state solutions, then they concentrate at one of these points

Solitary wave solution to the generalized nonlinear Schrodinger equation for dispersive permittivity and permeability

We present a solitary wave solution of the generalized nonlinear Schrodinger equation for dispersive permittivity and permeability using a scaling transformation and coupled amplitude-phase formulation. We have considered the third-order dispersion effect (TOD) into our model and show that soliton shift may be suppressed in a negative index material by a judicious choice of the TOD and self-steepening parameter.Comment: 6 page

Resonant nonlinear optics of backward waves in negative-index metamaterials

The extraordinary properties of resonant four-wave mixing of backward waves in doped negative-index materials are investigated. The feasibility of independent engineering of negative refractive index and nonlinear optical response as well as quantum control of the nonlinear propagation process in such composites is shown due to the coherent energy transfer from the control to the signal field. Laser-induced transparency, quantum switching, frequency-tunable narrow-band filtering, amplification, and realizing a miniature mirrorless optical parametric generator of the entangled backward and ordinary waves are among the possible applications of the investigated processes.Comment: 10 pages, 9 figure

Frequency-dependent (ac) Conduction in Disordered Composites: a Percolative Study

In a recent paper [Phys. Rev. B{\bf57}, 3375 (1998)], we examined in detail the nonlinear (electrical) dc response of a random resistor cum tunneling bond network ($RRTN$, introduced by us elsewhere to explain nonlinear response of metal-insulator type mixtures). In this work which is a sequel to that paper, we consider the ac response of the $RRTN$-based correlated $RC$ ($CRC$) model. Numerical solutions of the Kirchoff's laws for the $CRC$ model give a power-law exponent (= 0.7 near $p = p_c$) of the modulus of the complex ac conductance at moderately low frequencies, in conformity with experiments on various types of disordered systems. But, at very low frequencies, it gives a simple quadratic or linear dependence on the frequency depending upon whether the system is percolating or not. We do also discuss the effective medium approximation ($EMA$) of our $CRC$ and the traditional random $RC$ network model, and discuss their comparative successes and shortcomings.Comment: Revised and reduced version with 17 LaTeX pages plus 8 JPEG figure