Atomic coherence and interference phenomena in resonant nonlinear optical interactions

Interference effects in quantum transitions, giving rise to amplification without inversion, optical transparency and to enhancements in nonlinear optical frequency conversions are considered. Review of the relevant early theoretical and experimental results is given. The role of relaxation processes, spontaneous cascade of polarizations, local field effects, Doppler-broadening, as well as specific features of the interference in the spectral continuum are discussed.Comment: 13 pages, 13 eps figures, review paper, Proceedings of the 15th International Conference on Nonlinear Optics - ICONO'9

Accuracy of one-dimensional collision integral in the rigid spheres approximation

The accuracy of calculation of spectral line shapes in one-dimensional approximation is studied analytically in several limiting cases for arbitrary collision kernel and numerically in the rigid spheres model. It is shown that the deviation of the line profile is maximal in the center of the line in case of large perturber mass and intermediate values of collision frequency. For moderate masses of buffer molecules the error of one-dimensional approximation is found not to exceed 5%.Comment: LaTeX, 24 pages, 8 figure

New access to very weak interactions in molecules

It is predicted that nuclear spin conversion in molecules can be efficiently controlled by strong laser radiation resonant to rovibrational molecular transition. The phenomenon can be used for substantial enrichment of spin isomers, or for detection of very weak (10-100 Hz) interactions in molecules.Comment: REVTEX, 11 pages + 4 eps figure

Dressed-state amplification by a superconducting qubit

We demonstrate amplification of a microwave signal by a strongly driven two-level system in a coplanar waveguide resonator. The effect known from optics as dressed-state lasing is observed with a single quantum system formed by a persistent current (flux) qubit. The transmission through the resonator is enhanced when the Rabi frequency of the driven qubit is tuned into resonance with one of the resonator modes. Amplification as well as linewidth narrowing of a weak probe signal has been observed. The laser emission at the resonator's fundamental mode has been studied by measuring the emission spectrum. We analyzed our system and found an excellent agreement between the experimental results and the theoretical predictions obtained in the dressed-state model.Comment: 5 pages, 4 figure

Inversionless light amplification and optical switching controlled by state-dependent alignment of molecules

We propose a method to achieve amplification without population inversion by anisotropic molecules whose orientation by an external electric field is state-dependent. It is based on decoupling of the lower-state molecules from the resonant light while the excited ones remain emitting. The suitable class of molecules is discussed, the equation for the gain factor is derived, and the magnitude of the inversionless amplification is estimated for the typical experimental conditions. Such switching of the sample from absorbing to amplifying via transparent state is shown to be possible both with the aid of dc and ac control electric fields.Comment: AMS-LaTeX v1.2, 4 pages with 4 figure

Inversionless gain in a three-level system driven by a strong field and collisions

Inversionless gain in a three-level system driven by a strong external field and by collisions with a buffer gas is investigated. The mechanism of populating of the upper laser level contributed by the collision transfer as well as by relaxation caused by a buffer gas is discussed in detail. Explicit formulae for analysis of optimal conditions are derived. The mechanism developed here for the incoherent pump could be generalized to other systems.Comment: RevTeX, 9 pages, 4 eps figure