524 research outputs found
Resonant inelastic x-ray scattering in one-dimensional copper oxides
The Cu K-edge resonant inelastic x-ray scattering (RIXS) spectrum in
one-dimensional insulating cuprates is theoretically examined by using the
exact diagonalization technique for the extended one-dimensional
Hubbard model with nearest neighbor Coulomb interaction. We find the
following characteristic features that can be detectable by RIXS experiments:
(i) The spectrum with large momentum transfer indicates the formation of
excitons, i.e., bound states of holon and doublon. (ii) The spectrum with small
momentum transfer depends on the incident photon energy. We propose that the
RIXS provides a unique opportunity to study the upper
Hubbard band in one-dimensional cuprates.Comment: 3 pages with 4 figures, minor changes, to appear in Phys.Rev.
Spin correlations in the electron-doped high-transition-temperature superconductor Nd{2-x}Ce{x}CuO{4+/-delta}
High-transition-temperature (high-Tc) superconductivity develops near
antiferromagnetic phases, and it is possible that magnetic excitations
contribute to the superconducting pairing mechanism. To assess the role of
antiferromagnetism, it is essential to understand the doping and temperature
dependence of the two-dimensional antiferromagnetic spin correlations. The
phase diagram is asymmetric with respect to electron and hole doping, and for
the comparatively less-studied electron-doped materials, the antiferromagnetic
phase extends much further with doping [1, 2] and appears to overlap with the
superconducting phase. The archetypical electron-doped compound
Nd{2-x}Ce{x}CuO{4\pm\delta} (NCCO) shows bulk superconductivity above x \approx
0.13 [3, 4], while evidence for antiferromagnetic order has been found up to x
\approx 0.17 [2, 5, 6]. Here we report inelastic magnetic neutron-scattering
measurements that point to the distinct possibility that genuine long-range
antiferromagnetism and superconductivity do not coexist. The data reveal a
magnetic quantum critical point where superconductivity first appears,
consistent with an exotic quantum phase transition between the two phases [7].
We also demonstrate that the pseudogap phenomenon in the electron-doped
materials, which is associated with pronounced charge anomalies [8-11], arises
from a build-up of spin correlations, in agreement with recent theoretical
proposals [12, 13].Comment: 5 pages, 4 figure
Electronic Structure of Ladder Cuprates
We study the electronic structure of the ladder compounds (SrCa)CuO 14-24-41
and SrCuO 123. LDA calculations for both give similar Cu 3d-bands near the
Fermi energy. The hopping parameters estimated by fitting LDA energy bands show
a strong anisotropy between the t_perp t_par intra-ladder hopping and small
inter-ladder hopping. A downfolding method shows that this anisotropy arises
from the ladder structure.The conductivity perpendicular to the ladders is
computed assuming incoherent tunneling giving a value close to experiment.Comment: 5 pages, 3 figure
17O NMR study of q=0 spin excitations in a nearly ideal S=1/2 1D Heisenberg antiferromagnet, Sr2CuO3, up to 800 K
We used 17O NMR to probe the uniform (wavevector q=0) electron spin
excitations up to 800 K in Sr2CuO3 and separate the q=0 from the q=\pm\pi/a
staggered components. Our results support the logarithmic decrease of the
uniform spin susceptibility below T ~ 0.015J, where J=2200 K. From measurement
of the dynamical spin susceptibility for q=0 by the spin-lattice relaxation
rate 1/T_{1}, we demonstrate that the q=0 mode of spin transport is ballistic
at the T=0 limit, but has a diffusion-like contribution at finite temperatures
even for T << J.Comment: Submitted to Phys. Rev. Lett. 4 pages, 4 figure
Itinerancy and Hidden Order in
We argue that key characteristics of the enigmatic transition at in indicate that the hidden order is a density wave formed within
a band of composite quasiparticles, whose detailed structure is determined by
local physics. We expand on our proposal (with J.A. Mydosh) of the hidden order
as incommnesurate orbital antiferromagnetism and present experimental
predictions to test our ideas. We then turn towards a microscopic description
of orbital antiferromagnetism, exploring possible particle-hole pairings within
the context of a simple one-band model. We end with a discussion of recent
high-field and thermal transport experiment, and discuss their implications for
the nature of the hidden order.Comment: 18 pages, 7 figures. v2 contains added referenc
Cu-O network-dependent core-hole screening in low-dimensional cuprate systems: a high-resolution X-ray photoemission study
We present an experimental study of the dynamics of holes in the valence bands of zero-, one-, and two-dimensional undoped model cuprates, as expressed via the screening of a Cu 2p core hole. The response depends strongly upon the dimensionality and the details of the Cu-O-Cu network geometry and clearly goes beyond the present theoretical state-of-the-art description within the three-band d-p model
Momentum-Resolved Charge Excitations in a Prototype One Dimensional Mott Insulator
We report momentum resolved charge excitations in a one dimensional (1-D)
Mott insulator studied using high resolution (~ 325 meV) inelastic x-ray
scattering over the entire Brillouin zone for the first time. Excitations at
the insulating gap edge are found to be highly dispersive (momentum
dependent)compared to excitations observed in two dimensional Mott insulators.
The observed dispersion in 1-D is consistent with charge excitations involving
holons which is unique to spin-1/2 quantum chain systems. These results point
to the potential utility of inelastic x-ray scattering in providing valuable
information about electronic structure of strongly correlated insulators.Comment: 3 pages, 2 figures, Revised with minor change
Anisotropic spin freezing in the S=1/2 zigzag ladder compound SrCuO2
Using magnetic neutron scattering we characterize an unusual low temperature
phase in orthorhombic SrCuO2. The material contains zigzag spin ladders formed
by pairs of S=1/2 chains (J=180 meV) coupled through a weak frustrated
interaction |J'|<0.1J. At T<Tc1=5.0(4)K an elastic peak develops in a gapless
magnetic excitation spectrum indicating spin freezing on a time scale larger
than 200 picoseconds. While the frozen state has long range commensurate
antiferromagnetic order along the chains with the correlation length exceeding
200 lattice periods along the c-axis and a substantial correlation length of
60(25) spacings along the a-axis perpendicular to the zigzag plane, only 2
lattice units are correlated along the b-axis which is the direction of the
frustrated interactions. The frozen magnetic moment of each Cu ion is very
small, 0.033(7) Bohr magneton even at T=0.35K, and has unusual temperature
dependence with a cusp at Tc2=1.5K reminiscent of a phase transition. We argue
that slow dynamics of stripe-like cooperative magnetic defects in tetragonal
a-c planes yield this anisotropic frozen state.Comment: 4 pages, LaTeX, submitted to PR
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